Citation: Zeyu Zhu, Jing Zhu, Yangshen Chen, Xinxin Liu, Mengchun Zhang, Mengxiao Yang, Mengyu Liu, Jiansheng Wu, Sheng Li, Fengwei Huo. Leather waste as precursor to prepare bifunctional catalyst for alkaline and neutral zinc-air batteries[J]. Chinese Chemical Letters, ;2023, 34(6): 107756. doi: 10.1016/j.cclet.2022.107756 shu

Leather waste as precursor to prepare bifunctional catalyst for alkaline and neutral zinc-air batteries

Zeyu Zhu ^{a, 1} ,
Jing Zhu ^{a, 1} ,
Yangshen Chen ^{a, 1} ,
Xinxin Liu ^a ,
Mengchun Zhang ^b ,
Mengxiao Yang ^a ,
Mengyu Liu ^b ,
Jiansheng Wu ^{a, *,} ,
Sheng Li ^{a, *,} ,
Fengwei Huo ^{a, *,}

a.
Key Laboratory of Flexible Electronics (KLOFE), Institute of Advanced Materials (IAM), Nanjing Tech University, Nanjing 211816, China
b.
School of Chemistry and Molecular Engineering, Nanjing Tech University, Nanjing 211816, China

iamjswu@njtech.edu.cn

iamsli@njtech.edu.cn

iamfwhuo@njtech.edu.cn

Received Date: 6 May 2022
Revised Date: 26 May 2022
Accepted Date: 16 August 2022
Available Online: 19 August 2022

Figures(5)

Carbon materials derived from biomass waste are considered as potential electrocatalysts for applications in zinc-air batteries (ZABs) due to their low cost and good catalytic activity. Here, we reported the preparation of gel-based catalysts through utilizing hydrolyzed waste leather powder cross-linked with metallic salt solutions. After calcination, iron-nickel alloy anchored in nitrogen-doped porous carbon catalysts (FeNi@NDC) was achieved. Compared with commercial Pt/C catalyst, FeNi@NDC-800 exhibited lower E_1/2 (0.77 V) and better durability. More importantly, the resulting FeNi@NDC-800-based alkaline ZABs achieved power density of 93.01 mW/cm² and open circuit voltage of 1.45 V, which the FeNi@NDC-800-based neutral ZAB displayed a charge/discharge cycle stability of 275 h. This work opens up the possibility of rational design and preparation of low-cost and high-performance electrocatalysts from recyclable leather waste.
- Leather waste,
- Zinc-air batteries,
- Bifunctional electrocatalyst,
- FeNi alloy,
- Biomass
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