Citation: Jiafeng Zou, Wenwen Fei, Yao Qiao, Ying Yang, Zongbing He, Lei Feng, Man-Bo Li, Zhikun Wu. Combined synthesis of interconvertible Au₁₁Cd and Au₂₆Cd₅ for photocatalytic oxidations involving singlet oxygen[J]. Chinese Chemical Letters, ;2023, 34(4): 107660. doi: 10.1016/j.cclet.2022.07.003 shu

Combined synthesis of interconvertible Au₁₁Cd and Au₂₆Cd₅ for photocatalytic oxidations involving singlet oxygen

Jiafeng Zou ^{a, b} ,
Wenwen Fei ^{a, b, *,} ,
Yao Qiao ^{a, b} ,
Ying Yang ^{a, b} ,
Zongbing He ^{a, b} ,
Lei Feng ^{a, b} ,
Man-Bo Li ^{a, b, *,} ,
Zhikun Wu ^{a, b, *,}

a.
Institute of Physical Science and Information Technology, Anhui University, Hefei 230601, China
b.
Key Laboratory of Materials Physics, Anhui Key Laboratory of Nanomaterials and Nanotechnology, CAS Center for Excellence in Nanoscience, Institute of Solid State Physics, HFIPS, Chinese Academy of Sciences, Hefei 230031, China

wenwen.fei@ahu.edu.cn

mbli@ahu.edu.cn

zkwu@issp.ac.cn

Received Date: 19 March 2022
Revised Date: 14 June 2022
Accepted Date: 4 July 2022
Available Online: 6 July 2022

Figures(2)

A novel Au₁₁Cd nanocluster was synthesized by developing a combined method and controlling the kinetics, and another Au₂₆Cd₅ nanocluster was also obtained after the conditions were changed in the same reaction, which could transfer to Au₁₁Cd in a two-way style. Both alloy nanoclusters can photocatalyze the production of singlet oxygen (¹O₂) and exhibit enhanced efficiencies in photocatalyzing two kinds of organic oxidations involving singlet oxygen compared with their non-alloyed mother nanoclusters, indicating that the Cd-doping might be an efficient way to enhance the photocatalysis performance of gold nanoclusters and metal nanoclusters are promising photocatalysts for organic oxidation involving singlet oxygen.
- Gold nanoclusters,
- Cadmium-doping,
- Singlet oxygen,
- Photocatalysis,
- RLE-AGR
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通讯作者: 陈斌, bchen63@163.com

Combined synthesis of interconvertible Au₁₁Cd and Au₂₆Cd₅ for photocatalytic oxidations involving singlet oxygen