Citation: Zhen Wang, Jun-Yu Li, Tao Huang, Huai-Ming Li, Teng Zhang. A Cu-based metal-organic framework with two types of connecting nodes as catalyst for oxygen activation[J]. Chinese Chemical Letters, ;2023, 34(6): 107635. doi: 10.1016/j.cclet.2022.06.058 shu

A Cu-based metal-organic framework with two types of connecting nodes as catalyst for oxygen activation

Zhen Wang ^{a, b} ,
Jun-Yu Li ^{a, b} ,
Tao Huang ^a ,
Huai-Ming Li ^a ,
Teng Zhang ^{a, b, *,}

a.
State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou 350002, China
b.
University of Chinese Academy of Sciences, Beijing 100049, China

zhangteng@fjirsm.ac.cn

Received Date: 19 April 2022
Revised Date: 15 June 2022
Accepted Date: 21 June 2022
Available Online: 25 June 2022

Figures(2)

Using a ditopic organic linker 4-(1H-pyrazol-4-yl)benzoic acid (H₂pba), FICN-6, a metal-organic framework containing both Cu₂(O₂CR)₄ and Cu₃(OH)(pyz)₃(O₂CR) secondary building units (SBUs), was synthesized. FICN-6 adopts in an unusual intercatenated structure with SBUs from two distinct networks connecting to each other. Presence of Cu₃ clusters makes FICN-6 a good heterogeneous catalyst for oxygen activation and aerobic oxidative C-C coupling of organic boronic acids.
- Copper,
- Metal-organic framework,
- Oxidative C-C coupling,
- Oxygen activation,
- Boronic acids
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