Citation: Buke Wu, Yongbiao Mu, Zheng Li, Ming Li, Lin Zeng, Tianshou Zhao. Realizing high-voltage aqueous zinc-ion batteries with expanded electrolyte electrochemical stability window[J]. Chinese Chemical Letters, ;2023, 34(2): 107629. doi: 10.1016/j.cclet.2022.06.052 shu

Realizing high-voltage aqueous zinc-ion batteries with expanded electrolyte electrochemical stability window

Buke Wu ^{a, b, c, 1} ,
Yongbiao Mu ^{a, b, c, 1} ,
Zheng Li ^{a, b, c} ,
Ming Li ^d ,
Lin Zeng ^{a, b, c, *,} ,
Tianshou Zhao ^{a, b, c, *,}

a.
Shenzhen Key Laboratory of Advanced Energy Storage, Southern University of Science and Technology, Shenzhen 518055, China
b.
Department of Mechanical and Energy Engineering, Southern University of Science and Technology, Shenzhen 518055, China
c.
SUSTech Energy Institute for Carbon Neutrality, Southern University of Science and Technology, Shenzhen 518055, China
d.
State Key Laboratory of Advanced Technology for Materials Synthesis and Processing, Wuhan University of Technology, Wuhan 430070, China

zengl3@sustech.edu.cn

zhaots@sustech.edu.cn

Received Date: 8 May 2022
Revised Date: 28 May 2022
Accepted Date: 21 June 2022
Available Online: 27 June 2022

Figures(8)

Aqueous zinc-ion batteries (AZIBs) have aroused significant research interest around the world in the past decade. The use of low-cost aqueous electrolytes and a metallic Zn anode with a suitable redox potential and high energy density make AZIBs a potential alternative to commercial Li-ion batteries in the development of next-generation batteries. However, owing to the narrow electrochemical stability window (ESW) of aqueous electrolytes, the choice of cathode materials is limited, because of which AZIBs exhibit a relatively low operating voltage and energy density. Hence, expanding the ESW of aqueous electrolytes is important for the development of practical AZIBs. This paper systematically reviews the electrolyte engineering strategies being explored to broaden the ESW of AZIBs. An in-depth analysis of high-voltage AZIBs is also presented. We suggest that the realization of high-voltage AZIBs depends on the synergistic development of suitable electrolytes and cathode materials. In addition, the cost associated with their fabrication as well as the use of standardized electrochemical tests should be considered during the design of high-voltage AZIBs.
- High voltage,
- Aqueous zinc ion batteries,
- Electrolytes,
- Cathodes,
- Electrochemical stability window
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沈阳化工大学材料科学与工程学院沈阳 110142