Citation: Huayan Wang, Huixin Chen, Chi Chen, Miao Li, Yiming Xie, Xingcai Zhang, Xianwen Wu, Qiaobao Zhang, Canzhong Lu. Tea-derived carbon materials as anode for high-performance sodium ion batteries[J]. Chinese Chemical Letters, ;2023, 34(4): 107465. doi: 10.1016/j.cclet.2022.04.063 shu

Tea-derived carbon materials as anode for high-performance sodium ion batteries

Huayan Wang ^{a, b, 1} ,
Huixin Chen ^{b, f, 1} ,
Chi Chen ^{b, f} ,
Miao Li ^c ,
Yiming Xie ^{a, *,} ,
Xingcai Zhang ^{d, e} ,
Xianwen Wu ^g ,
Qiaobao Zhang ^{c, *,} ,
Canzhong Lu ^{b, f, **,}

a.
Engineering Research Center of Environment-Friendly Function Materials, Ministry of Education, Institute of Materials Physical Chemistry, Huaqiao University, Xiamen 361021, China
b.
CAS key Laboratory of Design and Assembly of Functional Nanostructures, and Fujian Provincial Key Laboratory of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou 350002, China
c.
Department of Materials Science and Engineering, College of Materials, Xiamen University, Xiamen 361005, China
d.
School of Engineering and Applied Sciences, Harvard University, Cambridge, MA 02138, United States
e.
School of Engineering, Massachusetts Institute of Technology, Cambridge, MA 02139, United States
f.
Xiamen Key Laboratory of Rare Earth Photoelectric Functional Materials, Xiamen Institute of Rare Earth Materials, Haixi Institutes, Chinese Academy of Sciences, Xiamen 361021, China
g.
School of Chemistry and Chemical Engineering, Jishou University, Jishou 416000, China

^**

ymxie@hqu.edu.cn

zhangqiaobao@xmu.edu.cn

czlu@fjirsm.ac.cn

Received Date: 17 March 2022
Revised Date: 21 April 2022
Accepted Date: 23 April 2022
Available Online: 29 April 2022

Figures(4)

Sodium-ion batteries (SIB) have attracted widespread attention in large-scale energy storage fields owing to the abundant reserve in the earth and similar properties of sodium to lithium. Biomass-based carbon materials with low-cost, controllable structure, simple processing technology, and environmental friendliness tick almost all the right boxes as one of the promising anode materials for SIB. Herein, we present a simple novel strategy involving tea tomenta biomass-derived carbon anode with enhanced interlayer carbon distance (0.44 nm) and high performance, which is constructed by N, P co-doped hard carbon (Tea-1100-NP) derived from tea tomenta. The prepared Tea-1100-NP composite could deliver a high reversible capacity (326.1 mAh/g at 28 mA/g), high initial coulombic efficiency (ICE = 90% at 28 mA/g), stable cycle life (262.4 mAh/g at 280 mA/g for 100 cycles), and superior rate performance (224.5 mAh/g at 1400 mA/g). Experimental results show that the excellent electrochemical performance of Tea-1100-NP due to the high number of active N, P-containing groups, and disordered amorphous structures provide ample active sites and increase the conductivity, meanwhile, large amounts of microporous shorten the Na⁺ diffusion distance as well as quicken ion transport. This work provides a new type of N, P co-doped high-performance tomenta-derived carbon, which may also greatly promote the commercial application of SIB.
- Tea tomenta,
- Co-doped,
- Hard carbon,
- Initial coulombic efficiency,
- Sodium-ion batteries
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