Citation: Changyuan Su, Zhixu Zhang, Jie Yao, Ming Chen, Peizhi Huang, Yi Zhang, Dawei Fu, Liyan Xie. Construction, photoelectric response and phase transition for new hybrid double perovskites showing narrow band gaps[J]. Chinese Chemical Letters, ;2023, 34(4): 107442. doi: 10.1016/j.cclet.2022.04.040 shu

Construction, photoelectric response and phase transition for new hybrid double perovskites showing narrow band gaps

Changyuan Su ^a ,
Zhixu Zhang ^a ,
Jie Yao ^a ,
Ming Chen ^{a, b} ,
Peizhi Huang ^b ,
Yi Zhang ^{a, c, *,} ,
Dawei Fu ^{b, *,} ,
Liyan Xie ^{b, *,}

a.
Ordered Matter Science Research Center, Jiangsu Key Laboratory for Science and Applications of Molecular Ferroelectrics, Southeast University, Nanjing 211189, China
b.
Institute for Science and Applications of Molecular Ferroelectrics, Key Laboratory of the Ministry of Education for Advanced Catalysis Materials, Zhejiang Normal University, Jinhua 321004, China
c.
Chaotic Matter Science Research Center, Department of Materials, Metallurgy and Chemistry, Jiangxi University of Science and Technology, Ganzhou 341000, China

yizhang1980@seu.edu.cn

dawei@seu.edu.cn

liyanxie@zjnu.edu.cn

Received Date: 7 March 2022
Revised Date: 29 March 2022
Accepted Date: 18 April 2022
Available Online: 20 April 2022

Figures(5)

To explore the lead-free key scientific issue in perovskite, double perovskite based on AgBi and CuBi was naturally selected as a competitive candidate due to its fascinating functional features, such as self-powered circularly polarized light detection, X-ray detection, photoluminescence and so on. However, the most challenging point is to simulate the structure and function of traditional lead-based perovskite in new double perovskite. At the same time, there are few suitable double perovskite systems with optical and electrical potential. The above two points greatly limit the competitiveness of double perovskite. In order to solve this problem, firstly, by analyzing and comparing previous studies, we used 2,2-dimethylpropan-1-aminium (abbreviated as 2,2-DPA) as the organic template to assemble materials. Solid-to-solid phase transition materials (2,2-DPA)₃Bi₂I₉ 1 and (2,2-DPA)₃Pb₂I₇ 2 were constructed. Along the path of lead-free and two-dimensional maintenance, we successfully synthesized (2,2-DPA)₄AgBiI₈·H₂O 3 and (2,2-DPA)₄CuBiI₈·H₂O 4. As two typical semiconductors, 3 and 4 with narrower optical band gaps of 1.98 and 1.76 eV show obvious photo-response when the xenon lamp with intensity of 20 mW/cm² is on or off, implying that they may be applied to light-harvesting and light-detecting devices. By referring to the phase transition mechanism of 1 and 2, 3 may be caused by ordered-disordered transition of the organic part, which was proven to be the first solid-to-solid phase transition material with <100> -oriented layered double perovskites with n = 1 by systematic characterization methods after dehydration for all we know. We believed that this work can provide meaningful guidance for the development of lead-free double perovskites.
- Double perovskite,
- Photoelectric response,
- Phase transition,
- Dielectric properties,
- Semiconducting behavior
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