Citation: Yi Ding, Lele Zhang, Xin Wang, Lina Han, Weike Zhang, Chunli Guo. Vanadium-based cathodes for aqueous zinc ion batteries: Structure, mechanism and prospects[J]. Chinese Chemical Letters, ;2023, 34(2): 107399. doi: 10.1016/j.cclet.2022.03.122 shu

Vanadium-based cathodes for aqueous zinc ion batteries: Structure, mechanism and prospects

College of Materials Science and Engineering, Taiyuan University of Technology, Taiyuan 030024, China

guochunli@tyut.edu.cn

Received Date: 18 December 2021
Revised Date: 14 February 2022
Accepted Date: 31 March 2022
Available Online: 3 April 2022

Figures(9)

As an emerging energy storage device with high-safety aqueous electrolytes, low-cost, environmental benignity and large-reserves, the rechargeable aqueous zinc-ion batteries (AZIBs) have attracted more and more attention. Vanadium-based compounds are also supposed as the potential candidate cathode materials for AZIBs due to their wide variety of phases, variable crystal structures and high theoretical capacity. In this review, the recent progress in the development of vanadium-based materials was summarized, and the relationship between the crystal structure types of active materials and Zn-ion transport mechanism was highlighted. During the charge-discharge process, the different electrostatic repulsion between the cations of vanadium-based compounds with different crystal structures and Zn²⁺ results in a variety of the Zn-ion storage mechanisms, which can be significant guidance for designing the advanced battery-electrode materials for AZIBs. Furthermore, other factors associated with the storage mechanisms, such as electrolyte components and electrode morphology, are discussed. Finally, the strategies to improve the electrical conductivity, inhibit the dissolution and stabilize the crystal structure of vanadium-based compounds are proposed and the future prospects for developing high-energy-density AZIBs are presented.
- Aqueous zinc ion batteries,
- Vanadium-based materials,
- Crystal structure,
- Storage mechanisms,
- Recent advances
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沈阳化工大学材料科学与工程学院沈阳 110142