Citation: Meihong Fan, Xiao Liang, Qiuju Li, Lili Cui, Xingquan He, Xiaoxin Zou. Boron: A key functional component for designing high-performance heterogeneous catalysts[J]. Chinese Chemical Letters, ;2023, 34(1): 107275. doi: 10.1016/j.cclet.2022.02.080 shu

Boron: A key functional component for designing high-performance heterogeneous catalysts

Meihong Fan ^a ,
Xiao Liang ^b ,
Qiuju Li ^c ,
Lili Cui ^a ,
Xingquan He ^{a, *,} ,
Xiaoxin Zou ^{b, *,}

a.
School of Chemistry and Environmental Engineering, Changchun University of Science and Technology, Changchun 130022, China
b.
State Key Laboratory of Inorganic Synthesis and Preparative Chemistry, College of Chemistry, Jilin University, Changchun 130012, China
c.
Department of Chemistry, College of Basic Medicine, Third Military Medical University (Army Medical University), Chongqing 400038, China

hexingquan@hotmail.com

xxzou@jlu.edu.cn

Received Date: 30 December 2021
Revised Date: 22 January 2022
Accepted Date: 27 February 2022
Available Online: 4 March 2022

Figures(10)

Heterogeneous catalysis is a vivid branch of traditional catalysis field, with the advantage of high efficiency and being easily separated from reactants and products after reaction, and have received widespread attentions in large-scale industrial production, especially in the field of energy utilization. Boron has been found to be a key functional component for designing high-performance heterogeneous catalysts. In this review, we cover and categorize the past and recent progress in boron-containing materials and their applications in heterogeneous catalysis particularly in energy‐related fields. The fundamental roles of boron components in the emerging heterogeneous catalysis of construction, regulation and stabilization of active phases/sites are highlighted, with the emphasis on how they regulating structural and electronic properties of host materials. We then categorize boron-containing catalysts into six kinds mainly including intermetallic boride catalysts, metal boride-derived catalysts, boron-doped catalysts, metal boride-decorated catalysts, boron-containing compounds as catalyst supports, and single-boron-site catalysts, as well as try to establish structure-catalytic activity relationship. The catalytic applications of these six boron-containing catalysts are discussed separately, focusing on the energy-related reactions such as hydrogen evolution reaction (HER), oxygen evolution reaction (OER), oxygen reduction reaction (ORR), carbon dioxide reduction reaction (CO₂RR) and nitrogen reduction reaction (NRR). Finally, the opportunities and challenges related to boron-containing compounds in the field of catalysis are prospected.
- Boron,
- Heterogeneous catalysis,
- Active site,
- Electronic structure,
- Structure-activity relationship
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沈阳化工大学材料科学与工程学院沈阳 110142