Citation: Ming Yue, Yajing Fu, Canping Zhang, Junxiao Fu, Shiquan Wang, Jianwen Liu. Dual-metal zeolite imidazolate framework for efficient lithium storage boosted by synergistic effects and self-assembly 2D nanosheets[J]. Chinese Chemical Letters, ;2022, 33(6): 3291-3295. doi: 10.1016/j.cclet.2021.12.015 shu

Dual-metal zeolite imidazolate framework for efficient lithium storage boosted by synergistic effects and self-assembly 2D nanosheets

Ming Yue ^a ,
Yajing Fu ^a ,
Canping Zhang ^a ,
Junxiao Fu ^a ,
Shiquan Wang ^{a, *,} ,
Jianwen Liu ^{a, b, *,}

a.
College of Chemistry and Chemical Engineering & Collaborative Innovation Center for Advanced Organic Chemical Materials Co-constructed by the Province and Ministry & Ministry of Educational Key Laboratory for the Synthesis and Application of Organic Functional Molecules, Hubei University, Wuhan 430062, China
b.
Jiangsu Pylon Battery Co., Ltd., Yangzhou 211400, China

wsqhao@hubu.edu.cn

jianwen@hubu.edu.cn

Received Date: 22 August 2021
Revised Date: 22 November 2021
Accepted Date: 6 December 2021
Available Online: 12 December 2021

Figures(4)

Metal-organic framework materials (MOFs), such as zeolitic imidazolate framework (ZIF), have been widely used in energy storage due to their advantages such as high structural stability, large specific surface, more active sites and skeleton structures. Herein, a novel two-dimensional (2D) CoCu-ZIF was synthesized by a facile solvothermal method. The as-prepared CoCu-ZIF nanosheets exhibit an ultrahigh reversible capacity of 2287.4 mAh/g and remains at 1172.1 mAh/g after 300 cycles at a current density of 100 mA/g, far better than that of the single Co-ZIF and Cu-ZIF. Additionally, the specific discharge capacity of CoCu-ZIF nanosheets can maintain at about 590 mAh/g after 1000 cycles at the current density of 2 A/g. Owing to the synergistic effect of two metals, function of nitrogen in the molecular and self-assembly 2D nanosheets, our research can provide strong support for the practical application of CoCu-ZIF materials in lithium ion batteries.
- Lithium ion batteries,
- Metal-organic frameworks,
- CoCu-ZIF nanosheets,
- Synergistic effect,
- Self-assembly
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