Citation: Jie Huang, Zhirong Liu, Dejuan Huang, Tianxiang Jin, Yong Qian. Electrochemical deposition of uranium oxide with an electrocatalytically active electrode using double potential step technique[J]. Chinese Chemical Letters, ;2022, 33(8): 3762-3766. doi: 10.1016/j.cclet.2021.11.008 shu

Electrochemical deposition of uranium oxide with an electrocatalytically active electrode using double potential step technique

Jie Huang ^a ,
Zhirong Liu ^{a, b} ,
Dejuan Huang ^b ,
Tianxiang Jin ^a ,
Yong Qian ^{a, b, *,}

a.
Jiangxi Province Key Laboratory of Polymer Micro/Nano Manufacturing and Devices, East China University of Technology, Nanchang 330013, China
b.
State Key Laboratory of Nuclear Resources and Environment, East China University of Technology, Nanchang 330013, China

yqianecit@163.com

Received Date: 7 August 2021
Revised Date: 16 September 2021
Accepted Date: 3 November 2021
Available Online: 10 November 2021

Figures(6)

The development of effective uranium-removal techniques is of great significance to the environment and human health. In this work, a double potential step technique (DPST) was applied to remove U(VI) from uranium-containing wastewater using a carbon felt electrode modified by graphene oxide/phytic acid composite (GO-PA@CF). The application of DPST can inhibit water splitting and prevent GO-PA from adsorbing other interfering ions in wastewater. The GO-PA composite can effectively accelerate the electrochemical reduction rate of U(VI), which significantly improved the electrochemical deposition rate of uranium oxide. As a result, the maximum removal efficiency and maximum removal capacity of GO-PA@CF electrode reached 98.7% and 1149.3 mg/g, respectively. The removal efficiency remained 97.2% after five cycles of reuse. Moreover, the removal efficiency of GO-PA@CF electrode can reach more than 70% in simulated wastewater.
- Electrochemical deposition,
- Uranium,
- Double potential step technique,
- Graphene oxide,
- Nanocomposites
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