Citation: Shilong Qin, Hanxun Zou, Yu Hai, Lei You. Aggregation-induced emission luminogens and tunable multicolor polymer networks modulated by dynamic covalent chemistry[J]. Chinese Chemical Letters, ;2022, 33(6): 3267-3271. doi: 10.1016/j.cclet.2021.11.001 shu

Aggregation-induced emission luminogens and tunable multicolor polymer networks modulated by dynamic covalent chemistry

Shilong Qin ^{a, b} ,
Hanxun Zou ^{b, *,} ,
Yu Hai ^b ,
Lei You ^{a, b, c, *,}

a.
College of Chemical Engineering, Fuzhou University, Fuzhou 350116, China
b.
State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou 350002, China
c.
Fujian Science & Technology Innovation Laboratory for Optoelectronic Information of China, Fuzhou 350108, China

zouhanxun@fjirsm.ac.cn

lyou@fjirsm.ac.cn

Received Date: 16 September 2021
Revised Date: 21 October 2021
Accepted Date: 1 November 2021
Available Online: 6 November 2021

Figures(4)

Aggregation-induced emission (AIE) based luminescent materials are generating intensive interest due to their unique fluorescence in the aggregation state. Herein we report a strategy of dynamic covalent chemistry (DCC) controlled AIE luminogens for the regulation of multicolor emission in reversible covalent polymer networks. Tetraphenylethene derived ring-chain tautomers were prepared, and the emission was readily controlled through multimode, such as changing the solvent, adding the base, and dynamic covalent reactions with amines. Moreover, the construction of dynamic covalent cross-linked luminescent hydrogels with tunable fluorescent, self-healing, and mechanical properties, was realized. The combination of AIE and aggregation-caused quenching (ACQ) fluorophores in the polymer network further enabled the realization of a multicolor modulator, including white emission, in both solution and gel states. The strategies and results presented should find utility in dynamic assemblies, polymer networks, chemical sensing, and responsive materials.
- Aggregation-induced emission,
- Dynamic covalent chemistry,
- Stimuli-responsive materials,
- Covalent polymer network,
- Multicolor emission
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