Citation: Lele Lu, Qiang Li, Jia Du, Wei Shi, Peng Cheng. Bimetallic cobalt-nickel coordination polymer electrocatalysts for enhancing oxygen evolution reaction[J]. Chinese Chemical Letters, ;2022, 33(6): 2928-2932. doi: 10.1016/j.cclet.2021.10.090 shu

Bimetallic cobalt-nickel coordination polymer electrocatalysts for enhancing oxygen evolution reaction

Department of Chemistry, Key Laboratory of Advanced Energy Materials Chemistry (MOE), Renewable Energy Conversion and Storage Center (RECAST), College of Chemistry, Nankai University, Tianjin 300071, China

shiwei@nankai.edu.cn

Received Date: 30 July 2021
Revised Date: 16 September 2021
Accepted Date: 28 October 2021
Available Online: 5 November 2021

Figures(6)

Coordination polymers (CPs) have great potential to be used in electrocatalysis owing to their designable compositions and structures. It is highly challenging to apply CPs as electrocatalysts for oxygen evolution reaction (OER) on account of insufficient catalytic efficiency and relatively poor stability of current electrocatalysts. Herein, through a mixed-metal strategy, one-dimensional CoNi_1--HIPA with dual active sites was synthesized and studied for OER electrocatalysts. By changing the metal ratio of CoNi_1--HIPA, the OER performance was well regulated. The optimized Co_1/2Ni_1/2-HIPA exhibited minimum reaction activation energy, and represented an overpotential of 367 mV to reach 10 mA/cm² at 25 ℃. Moreover, an overpotential of 314 mV at 10 mA/cm² was obtained from Co_1/2Ni_1/2-HIPA at 55 ℃. This mixed-metal strategy provides a feasible way for adjusting the electronic states of the electrocatalysts to improve the electrocatalytic OER performance.
- Coordination polymer,
- Mixed-metal strategy,
- Electrocatalysis,
- Oxygen evolution reaction,
- Activation energy
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