Citation: Yi Zhou, Jialai Hu, Lichun Yang, Qingsheng Gao. Recent advances of two-dimensional CoFe layered-double-hydroxides for electrocatalytic water oxidation[J]. Chinese Chemical Letters, ;2022, 33(6): 2845-2855. doi: 10.1016/j.cclet.2021.10.034 shu

Recent advances of two-dimensional CoFe layered-double-hydroxides for electrocatalytic water oxidation

Yi Zhou ^{a, c} ,
Jialai Hu ^a ,
Lichun Yang ^{b, *,} ,
Qingsheng Gao ^{a, *,}

a.
College of Chemistry and Materials Science, and Guangdong Provincial Key Laboratory of Functional Supramolecular Coordination Materials and Applications, Jinan University, Guangzhou 510632, China
b.
School of Materials Science and Engineering, and Guangdong Provincial Key Laboratory of Advanced Energy Storage Materials, South China University of Technology, Guangzhou 510640, China
c.
Ningbo Fengcheng Advanced Energy Materials Research Institute Co., Ltd., Ningbo 315000, China

mslcyang@scut.edu.cn

tqsgao@jnu.edu.cn

Received Date: 30 August 2021
Revised Date: 26 September 2021
Accepted Date: 15 October 2021
Available Online: 21 October 2021

Figures(9)

Oxygen evolution reaction (OER) is pivotal to drive green hydrogen generation from water electrolysis, but yet is strictly overshadowed by the sluggish reaction kinetics. Earth-abundant and cut-price transition-metal compounds, particularly CoFe layered-double-hydroxides (LDHs), show the distinct superiorities in contrast to noble metals and their derivatives. In this review, we firstly underline their fundamental issues in electrocatalytic water oxidation, including CoFe LDHs crystal structure, the surface of (hydr)oxides confined to OER and the controversial roles of Fe species, aiming at understanding the structure-related activity and catalytic mechanism. Advanced approaches for optimizing OER activity of CoFe LDHs are then comprehensively overviewed, which will shed light on the different working mechanisms and provide a concise analysis of their unique advantages. Finally, a perspective on the future development of CoFe LDHs electrocatalysts is offered. We hope this review can give a concise and explicit guidance for the development of transition-metal-based electrocatalysts in the energy field.
- CoFe layered-double-hydroxides,
- Electrocatalytic water oxidation,
- Two-dimensional nanostructures,
- Surface reconstruction,
- d-band
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沈阳化工大学材料科学与工程学院沈阳 110142