Citation: Xiaoyan Li, Xiaoqin Liu, Yu Xiang, Qiaoji Zheng, Xijun Wei, Dunmin Lin. Metal-organic frameworks derived carbon-coated ZnSe/Co_0.85Se@N-doped carbon microcuboid as an advanced anode material for sodium-ion batteries[J]. Chinese Chemical Letters, ;2022, 33(6): 3197-3202. doi: 10.1016/j.cclet.2021.10.014 shu

Metal-organic frameworks derived carbon-coated ZnSe/Co_0.85Se@N-doped carbon microcuboid as an advanced anode material for sodium-ion batteries

Xiaoyan Li ^a ,
Xiaoqin Liu ^a ,
Yu Xiang ^a ,
Qiaoji Zheng ^a ,
Xijun Wei ^{b, *} ,
Dunmin Lin ^{a, *}

a.
College of Chemistry and Materials Science, Sichuan Normal University, Chengdu 610066, China
b.
State Key Laboratory of Environment-Friendly Energy Materials, School of Materials Science and Engineering, Southwest University of Science and Technology, Mianyang 621010, China

xijunwei1992@swust.edu.cn

ddmd222@sicnu.edu.cn

Received Date: 15 July 2021
Revised Date: 29 September 2021
Accepted Date: 8 October 2021
Available Online: 14 October 2021

Figures(5)

Transition metal selenides attract significant attention as advanced anode materials for sodium-ion batteries (SIBs) in recent years due to their appropriate working potential and high theoretic capacity. However, the poor structural stability and rate capability limit their further practical applications. Herein, zeolite imidazole framework-8/zeolite imidazole framework-67 is used as a template to prepare Co_0.85Se and ZnSe nanoparticles embed in N-doped carbon matrix successfully, and then coated a carbon layer (ZCS@NC@C) by in-situ polymerization. One side, the N-doped carbon matrix with rich pore structure not only shorten the diffusion path of Na⁺ and improve the conductivity of the electrode, but also prevent structural collapse and agglomeration of active particles during the sodium insertion/extraction process. On the other side, the carbon shell preparation by coating can form a protective layer to buffer the volumetric stress generated in the electrochemical process and further improve the electrical conductivity. As a result, the as-prepared ZCS@NC@C anode material exhibits an excellent electrochemical performance for SIBs. This investigation provides a promising approach to optimize the electrochemical performance of SIBs by incorporating active metal compounds into conductive carbons to form multidimensional structure.
- Transition metal selenides,
- N-doped,
- ZIF-8/ZIF-67,
- Carbon coating,
- Sodium ion batteries
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沈阳化工大学材料科学与工程学院沈阳 110142

Metal-organic frameworks derived carbon-coated ZnSe/Co0.85Se@N-doped carbon microcuboid as an advanced anode material for sodium-ion batteries

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通讯作者: 陈斌, bchen63@163.com

Metal-organic frameworks derived carbon-coated ZnSe/Co_0.85Se@N-doped carbon microcuboid as an advanced anode material for sodium-ion batteries