Citation: Yuxuan Ye, Peng Yang, Yuwei Deng, Yezhi Yang, Kun Zhang, Yueying Wang, Wenjing Shang, Qiang Li, Lei Sun, Fei Pan, Dongsheng Xia. Non-woven cotton fabric based intimately coupling of photocatalysis and biodegradation system for efficient removal of Cu(Ⅱ) complex in water[J]. Chinese Chemical Letters, ;2022, 33(6): 3127-3132. doi: 10.1016/j.cclet.2021.10.009 shu

Non-woven cotton fabric based intimately coupling of photocatalysis and biodegradation system for efficient removal of Cu(Ⅱ) complex in water

Yuxuan Ye ^{a, b} ,
Peng Yang ^a ,
Yuwei Deng ^a ,
Yezhi Yang ^a ,
Kun Zhang ^a ,
Yueying Wang ^a ,
Wenjing Shang ^a ,
Qiang Li ^{a, b} ,
Lei Sun ^a ,
Fei Pan ^{a, b, *,} ,
Dongsheng Xia ^{a, b, *,}

a.
School of Environmental Engineering, Wuhan Textile University, Wuhan 430073, China
b.
Engineering Research Center for Clean Production of Textile Dyeing and Printing, Ministry of Education, Wuhan 430073, China

fpan@wtu.edu.cn

dongsheng_xia@wtu.edu.cn

Received Date: 17 July 2021
Revised Date: 16 August 2021
Accepted Date: 8 October 2021
Available Online: 14 October 2021

Figures(5)

The efficient remediation of heavy metal complexes in water has become a difficult and challenging task owing to their high stability and strong mobility. In this study, a novel strategy was employed for highly efficient removal of Cu-citrate by using intimately coupled photocatalysis and biodegradation (ICPB) system with non-woven cotton fabric as a carrier. Experimental results showed that the ICPB system caused 94% Cu removal, which was higher than those of single photocatalysis. After 5 cycles, Cu removal efficiency could still reach 78% within 5 h. The existence of 0–40 mg/L citrate had negligible influence, whereas the presence of 60–100 mg/L citrate exhibited a limited adverse effect on Cu removal (~70%). The decomplexation of Cu-citrate was realized via the function of free radicals and microorganisms. Two main processes, such as bio-adsorption of Cu²⁺ by microorganisms, deposition of Cu⁰ on the surface of material, played important role in Cu removal from aqueous solution. The dominant microorganisms in the system were Proteobacteria, Actinobacteria, Bacteroidetes, Chloroflexi, Chlorophyta, Planctomycetes, and Verrucomicrobia. Furthermore, the performance of ICPB system was also validated through treatment of other heavy metal complexes. This study provided a feasible strategy for the decontamination of heavy metal complexes in wastewater.
- Cu complex,
- Photocatalysis,
- Biological treatment,
- Non-woven cotton fabric
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沈阳化工大学材料科学与工程学院沈阳 110142