Citation: Weirui Qian, Minzan Zuo, Pengbo Niu, Xiao-Yu Hu, Leyong Wang. The construction of aggregation-induced charge transfer emission systems in aqueous solution directed by supramolecular strategy[J]. Chinese Chemical Letters, ;2022, 33(4): 1975-1978. doi: 10.1016/j.cclet.2021.09.070 shu

The construction of aggregation-induced charge transfer emission systems in aqueous solution directed by supramolecular strategy

Weirui Qian ^a ,
Minzan Zuo ^b ,
Pengbo Niu ^a ,
Xiao-Yu Hu ^{b, *,} ,
Leyong Wang ^{a, c, *,}

a.
Key Laboratory of Mesoscopic Chemistry of MOE, Jiangsu Key Laboratory of Advanced Organic Materials, School of Chemistry and Chemical Engineering, Nanjing University, Nanjing 210023, China
b.
College of Materials Science and Technology, Nanjing University of Aeronautics and Astronautics, Nanjing 211106, China
c.
Department of Chemistry, Xihua University, Chengdu 610039, China

huxy@nuaa.edu.cn

lywang@nju.edu.cn

Received Date: 3 August 2021
Revised Date: 18 September 2021
Accepted Date: 22 September 2021
Available Online: 26 September 2021

Figures(5)

Novel aggregation-induced charge transfer (CT) emission systems with long luminescence lifetime directed by supramolecular strategy have been successfully developed in water. The dimethylacridine-based electron donor (BrAc) with excellent aggregation ability can co-aggregate with a triazine-based electron acceptor (TRZ) to form nanorods in water, which exhibit CT emission with long lifetime (τ = 0.92 µs). As for a similar electron donor (QaAc) with poor aggregation ability, water-soluble pillar[5]arene (WP5) can be introduced to promote the aggregation process, leading to the obvious CT emission with long lifetime (τ = 0.61 µs). In addition, structural modification of the acceptor with substituent groups possessing stronger electron-accepting capabilities will cause red-shift (about 50 nm) of the emission, which allows conveniently constructing long lifetime organic luminescent materials with different emission colors.
- Aggregation-induced charge transfer emission,
- Supramolecular strategy,
- Long luminescence lifetime,
- Self-assemble,
- Co-aggregate
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