Citation: Hongyang Chen, Manxian Li, Chuanping Li, Xuan Li, Yaling Wu, Xiaochuan Chen, Junxiong Wu, Xiaoyan Li, Yuming Chen. Electrospun carbon nanofibers for lithium metal anodes: Progress and perspectives[J]. Chinese Chemical Letters, ;2022, 33(1): 141-152. doi: 10.1016/j.cclet.2021.08.097 shu

Electrospun carbon nanofibers for lithium metal anodes: Progress and perspectives

Hongyang Chen ^{a, 1} ,
Manxian Li ^{a, 1} ,
Chuanping Li ^a ,
Xuan Li ^a ,
Yaling Wu ^{b, *,} ,
Xiaochuan Chen ^{c, *,} ,
Junxiong Wu ^{a, *,} ,
Xiaoyan Li ^a ,
Yuming Chen ^{a, d, **,}

a.
College of Environmental Science and Engineering, Fujian Normal University, Fuzhou 350007, China
b.
College of Life Science, Fujian Normal University, Fuzhou 350007, China
c.
School of Chemistry, Sun Yat-Sen University, Guangzhou 510275, China
d.
State Key Laboratory of Structural Chemistry, Fuzhou 350000, China

yaling_wu@outlook.com

chenxch29@126.com

jwuba@connect.ust.hk

yumingc126@126.com

Received Date: 9 August 2021
Revised Date: 16 August 2021
Accepted Date: 21 August 2021
Available Online: 26 August 2021

Figures(8)

Li metal anodes (LMAs) has attracted extensive research interest because of its extremely high theoretical capacity (3860 mAh/g) at low redox potential (−3.04 V vs. standard hydrogen electrode). However, the extremely high chemical reactivity and the intrinsic "hostless" nature of LMAs bring about serious dendritic growth and dramatic volume change during the plating/strapping process, thus resulting in poor Coulombic efficiency, short lifespan, and severe safety concerns. Of various strategies, the construction of three-dimensional carbonaceous scaffolds for LMAs can substantially reduce the local current density, inhibit Li dendrite growth, and accommodate volume variation. Electrospinning is a simple yet effective strategy to fabricate carbon nanofibers (CNFs), which have been regarded as promising skeletons for LMAs, owing to their large surface areas, good electrical conductivity, and high porosity. In this Mini Review, we briefly introduce the fabrication of CNFs using electrospinning and the modification of CNFs. We highlight the recent advances in electrospun CNF skeletons for LMAs, including pure CNF and CNF-based composite scaffolds. Finally, we discuss the remaining challenges of electrospun CNF scaffolds for LMAs and provide possible solutions to push forward the advancement in this field.
- Electrospinning,
- Lithium metal anodes,
- Carbon nanofibers,
- Lithiophilic hosts,
- Three-dimensional skeletons
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沈阳化工大学材料科学与工程学院沈阳 110142