Citation: Xiaojun Zhang, Xiaomeng Jin, Yuxin Li. Water-induced luminescence improvement in a lanthanide β-diketone complex for monitoring water purity[J]. Chinese Chemical Letters, ;2022, 33(4): 2117-2120. doi: 10.1016/j.cclet.2021.08.080 shu

Water-induced luminescence improvement in a lanthanide β-diketone complex for monitoring water purity

Key Laboratory of Function Inorganic Material Chemistry (MOE), School of Chemistry and Material Science, Heilongjiang University, Harbin 150080, China

liyuxin@hlju.edu.cn

Received Date: 29 May 2021
Revised Date: 7 August 2021
Accepted Date: 17 August 2021
Available Online: 21 August 2021

Figures(4)

Water-caused luminescence quenching is a well-known and intractable issue for luminescence lanthanide complexes, greatly confining their broad application as sensing and displaying devices in water system. Herein, an anionic and coordination-saturated lanthanide complex with a nanosheet-like structure has been prepared. It exhibits excellent photophysical properties both in solid state and in aqueous suspension. Noteworthily, a 13% improvement for sensitization efficiency from organic ligand to central lanthanide ion has been realized, indicating an exceptional phenomenon of water-induced luminescence improvement which is rarely reported previously. Moreover, the aqueous suspension of as-prepared luminophore could act as a chemo-sensor responding to various organic solvents in water. Both of water-induced luminescence improvement and extended sensing behavior in this work provide a new platform for developing highly performant and practical luminescent materials in the water system.
- Water-induced luminescence improvement,
- Lanthanide complex,
- β-Diketone ligand,
- Water quality monitor,
- Luminescence sensing,
- Through-space charge transfer
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