Citation: Chun Sun, Mingming Liu, Longlu Wang, Lingbin Xie, Weiwei Zhao, Jianmin Li, Shujuan Liu, Dafeng Yan, Qiang Zhao. Revisiting lithium-storage mechanisms of molybdenum disulfide[J]. Chinese Chemical Letters, ;2022, 33(4): 1779-1797. doi: 10.1016/j.cclet.2021.08.052 shu

Revisiting lithium-storage mechanisms of molybdenum disulfide

Chun Sun ^a ,
Mingming Liu ^a ,
Longlu Wang ^{a, *,} ,
Lingbin Xie ^b ,
Weiwei Zhao ^b ,
Jianmin Li ^a ,
Shujuan Liu ^b ,
Dafeng Yan ^c ,
Qiang Zhao ^{a, b, *,}

a.
College of Electronic and Optical Engineering & College of Microelectronics, Institute of Flexible Electronics (Future Technology), Nanjing University of Posts & Telecommunications (NUPT), Nanjing 210023, China
b.
Key Laboratory for Organic Electronics and Information Displays & Jiangsu Key Laboratory for Biosensors, Institute of Advanced Materials (IAM), Nanjing University of Posts & Telecommunications, Nanjing 210023, China
c.
College of Chemistry and Environmental Engineering, Shenzhen University, Shenzhen 518060, China

wanglonglu@hnu.edu.cn

iamqzhao@njupt.edu.cn

Received Date: 17 June 2021
Revised Date: 10 July 2021
Accepted Date: 11 August 2021
Available Online: 16 August 2021

Figures(18)

Molybdenum disulfide (MoS₂), a typical two-dimensional transition metallic layered material, attracts tremendous attentions in the electrochemical energy storage due to its excellent physicochemical properties. However, with the deepening of the research and exploration of the lithium storage mechanism of these advanced MoS₂-based anode materials, the complex reaction process influenced by internal and external factors hinders the exhaustive understanding of the lithium storage process. To design stable anode material with high performance, it is urgent to review the mechanisms of reported anode materials and summarize the related factors that influence the reaction processes. This review aims to dissect all possible side reactions during charging and discharging process, uncover internal and external factors inducing various anode reactions and finally put forward strategies of controlling high cycling capacity and super-stable lithium storage capability of MoS₂. This review will be helpful to the design of MoS₂-based lithium-ion batteries (LIBs) with excellent cycle performance to enlarge the application fields of these advanced electrochemical energy storage devices.
- Lithium-ion batteries,
- Molybdenum disulfide (MoS₂),
- Lithium storage mechanisms,
- MoS₂-based anode materials,
- In situ characterization methods
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沈阳化工大学材料科学与工程学院沈阳 110142