Citation: Nkongolo Tshamala Aristote, Kangyu Zou, Andi Di, Wentao Deng, Baowei Wang, Xinglan Deng, Hongshuai Hou, Guoqiang Zou, Xiaobo Ji. Methods of improving the initial Coulombic efficiency and rate performance of both anode and cathode materials for sodium-ion batteries[J]. Chinese Chemical Letters, ;2022, 33(2): 730-742. doi: 10.1016/j.cclet.2021.08.049 shu

Methods of improving the initial Coulombic efficiency and rate performance of both anode and cathode materials for sodium-ion batteries

a.
College of Chemistry and Chemical Engineering, Central South University, Changsha 410083, China
b.
Department of Materials and Environmental Chemistry, Stockholm University, Stockholm 10691, Sweden

Author Bio: Nkongolo Tshamala Aristote is a master candidate at the College of Chemistry and Chemical Engineering, Central South University (China). He received B. Sc from the Polytechnics Faculty, Department of Metallurgical Engineering, University of Lubumbashi (D.R. Congo) in 2017. His research focuses on the construction of hard carbon as high initial coulombic efficiency and rate performance anode material for sodium-ion batteries.
Kangyu Zou is a Ph.D. candidate at the College of Chemistry andChemical Engineering, Central South University. He received his B.Sc. and M.Sc. degrees from Northwest University (Xi’an, China) in 2015 and 2018, respectively. His research is focused on the construction of highperformance metal ion capacitors.
Dr. Andi Di is currently a research fellow at Stockholm University, Stockholm, Sweden. She received master degree at Harbin Institute of Technology, and got Ph.D at University of Bath supervised by Prof. Karen Edler. Then she undertook postdoc work with Prof. Lennart Bergström at Stockholm University as a research fellow.
Dr. Wentao Deng is currently a research fellow at Central South University, Changsha, China. She received master degree with the supervision of Prof. Xiaobo Ji at Central South University, and got Ph.D at University of Bath supervised by Dr. Petra Cameron. Then she undertook postdoc work with Prof. Laurie Peter at University of Bath before joining Central South University as a research fellow.
Baowei Wang is a master candidate of College of Chemistry and Chemical Engineering, Central South University. He received his B.S. degree from China University of Mining and Technology in 2019. His research interests focus on the development of Nb-based materials for sodium-ion capacitors.
Xinglan Deng is a master candidate of College of Chemistry and Chemical Engineering, Central SouthUniversity. She received her B.S. degreefrom Xiangtan University in 2019. Her research isfocused on the development of novel electrode materials for sodium ion capacitors.
Hongshuai Hou is an Associate Professor at the College of Chemistry and Chemical Engineering, Central South University. He received his Ph.D. at Central South University in 2016. His current research interests are electrochemistry and key materials for electrochemical energy storage devices.
Guoqiang Zou is an associate professor at the College of Chemistry and Chemical Engineering, Central South University. He received his Ph.D. from Central SouthUniversity in 2018. His current research interests are electrochemistry and key materials for electrochemical energy storage devices.
Xiaobo Ji is a "Shenghua" Professor at Central South University and a Fellow of the Royal Society of Chemistry, specializing in the research and development of batteries and supercapacitor materials and their systems. He received his PhD in Electrochemistry in 2007 under the supervisionof Prof. Richard Compton at the University of Oxford and undertook postdoctoral work at MIT with Prof. Donald Sadoway.

gq-zou@csu.edu.cn

Received Date: 31 May 2021
Revised Date: 12 July 2021
Accepted Date: 11 August 2021
Available Online: 17 August 2021

Figures(12)

Sodium-ion batteries (SIBs) have gained more scientists' interest, owing to some facts such as the natural abundance of Na, the similarities of physicochemical characteristics between Li and Na. The irreversible Na⁺ ions consumption during the first cycle of charge/discharge process (due to the formation of the solid electrolyte interface (SEI) on the electrode surface and other irreversible reactions) is the factor that determines high performance SIBs and largely reduces the capacity of the full cell SIBs. Thus, the initial coulombic efficiency (ICE) of SIBs for both anode and cathode materials, is a key parameter for high performance SIBs, and the point is to increase the transport rate of the Na⁺ ions. Therefore, developing SIBs with high ICE and rate performance becomes vital to boost the commercialization of SIBs. Here we provide a review on the methods to improve the ICE and the rate performance, by summarizing some methods of improving the ICE and rate performance of the anode and cathode materials for SIBs, and end by a conclusion with some perspectives and recommendations.
- Initial coulombic efficiency,
- Rate performance,
- Sodium-ion batteries,
- Anode materials,
- Cathode materials
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