Citation: Danni Guo, Lixia Zhao, Hui Zhang. Crystallinity engineering of Au nanoparticles on graphene for in situ SERS monitoring of Fenton-like reaction[J]. Chinese Chemical Letters, ;2022, 33(3): 1263-1266. doi: 10.1016/j.cclet.2021.07.051 shu

Crystallinity engineering of Au nanoparticles on graphene for in situ SERS monitoring of Fenton-like reaction

Danni Guo ^{a, b} ,
Lixia Zhao ^{a, *,} ,
Hui Zhang ^{a, c, *,}

a.
State Key Laboratory of Environmental Chemistry and Eco-toxicology, Research Center for Eco-environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China
b.
College of Resources and Environment, University of Chinese Academy of Sciences, Beijing 100049, China
c.
State Key Laboratory of Water Environment Simulation, School of Environment, Beijing Normal University, Beijing 100875, China

zlx@rcees.ac.cn

zhanghui@bnu.edu.cn

Received Date: 6 May 2021
Revised Date: 4 June 2021
Accepted Date: 22 July 2021
Available Online: 31 July 2021

Figures(5)

Fabrication of multifunctional nanoplatform to in situ monitor Fenton reaction is of vital importance to probe the underlying reaction process and design high-performance catalyst. Herein, a hybrid catalyst comprising of single-crystalline Au nanoparticles (SC Au NPs) on reduced graphene oxide (RGO) sheet was prepared, which not only exhibited an excellent ¹O₂ mediated Fenton-like catalytic activity in promoting rhodamine 6G (R6G) degradation by activating H₂O₂, but also displayed a sensitive surface-enhanced Raman spectroscopy (SERS) detection performance to R6G with a linear response range from 1.0 × 10^-8 mol/L to 1.0 × 10^-5 mol/L thus providing a powerful and versatile nanoplatform for in situ SERS monitoring Fenton-like catalytic reaction. The integration of catalytic and SERS activities into a single nanostructure are expected to provide great potentials for practical applications in environmental catalysis.
- Au nanoparticle,
- Crystallinity engineering,
- Fenton-like reaction,
- SERS monitoring,
- Environmental remediation
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