Citation: Xiaowan Zhang, Yixin Yang, Peige Qin, Lizhen Han, Wenli Zhu, Shaofeng Duan, Minghua Lu, Zongwei Cai. Facile preparation of nano-g-C₃N₄/UiO-66-NH₂ composite as sorbent for high-efficient extraction and preconcentration of food colorants prior to HPLC analysis[J]. Chinese Chemical Letters, ;2022, 33(2): 903-906. doi: 10.1016/j.cclet.2021.07.003 shu

Facile preparation of nano-g-C₃N₄/UiO-66-NH₂ composite as sorbent for high-efficient extraction and preconcentration of food colorants prior to HPLC analysis

Xiaowan Zhang ^a ,
Yixin Yang ^a ,
Peige Qin ^a ,
Lizhen Han ^a ,
Wenli Zhu ^a ,
Shaofeng Duan ^b ,
Minghua Lu ^{a, *,} ,
Zongwei Cai ^c

a.
Henan International Joint Laboratory of Medicinal Plants Utilization, School of Chemistry and Chemical Engineering, Henan University, Kaifeng 475004, China
b.
Institute for Innovative Drug Design and Evaluation, School of Pharmacy, Henan University, Kaifeng 475004, China
c.
State Key Laboratory of Environmental and Biological Analysis, Department of Chemistry, Hong Kong Baptist University, Hong Kong, China

mhlu@henu.edu.cn

Received Date: 12 April 2021
Revised Date: 27 June 2021
Accepted Date: 1 July 2021
Available Online: 8 July 2021

Figures(4)

In this work, the nano-g-C₃N₄/UiO-66-NH₂ composite was prepared by one-step solvothermal method. The as-prepared composite was characterized by scanning electron microscopy, Brunner-Emmet-Teller measurement, energy dispersive spectrometer, X-ray diffraction, and Fourier transform infrared spectroscopy. By using nano-g-C₃N₄/UiO-66-NH₂ composite as sorbent, a dispersive solid-phase extraction coupled with high-performance liquid chromatography was developed to sensitive analysis of food colorants including tartrazine, amaranth, carmine, sunset yellow, allura red and bright blue. The experiment parameters including the amount of sorbent, adsorption time, the pH of adsorption solution, desorption time, desorption solvent, the pH of desorption solution as well as the proportion between desorption solvent and buffer solvent were investigated. Under the optimized conditions, the limits of detection (S/N = 3) and limits of quantitation (S/N = 10) were determined in the ranges of 0.08–0.8 and 0.2–2.0 ng/mL, respectively. With the developed sample pretreatment method, carmine and brilliant blue were determined from blueberry juice by HPLC-DAD. The contents were calculated as 1.53 µg/mL and 0.17 µg/mL, respectively.
- Nano-g-C₃N₄/UiO-66-NH₂ composite,
- Metal-organic frameworks,
- Dispersive solid-phase extraction,
- Sample pretreatment,
- Food colorants,
- Food additives,
- High-performance liquid chromatography
1. [1]
  W.L. Wu, S.Y. Liu, T.R. Guo, et al., Food Chem.356 (2021) 129643. doi: 10.1016/j.foodchem.2021.129643
2. [2]
  R. Różyło, Trends Food Sci. Technol. 102 (2020) 39–50. doi: 10.1016/j.tifs.2020.06.005
3. [3]
  S. Mathiyalagan, B.K. Mandal, Y.C. Ling, Food Chem. 278 (2019) 381–387. doi: 10.1016/j.foodchem.2018.11.077
4. [4]
  P. Amchova, H. Kotolova, J. Ruda-Kucerova, Regul. Toxicol. Pharmacol. 73 (2015) 914–922. doi: 10.1016/j.yrtph.2015.09.026
5. [5]
  G. Karanikolopoulos, A. Gerakis, K. Papadopoulou, et al., Food Chem. 177 (2015) 197–203. doi: 10.1016/j.foodchem.2015.01.026
6. [6]
  N. Pandey, R. Jain, A. Pandey, et al., Mycology9 (2018) 81–92. doi: 10.1080/21501203.2017.1423127
7. [7]
  P.M. Nowak, J. Chromatogr. A 1620 (2020) 460976.
8. [8]
  S. Jampasa, W. Siangproh, K. Duangmal, et al., Talanta160 (2016) 113–124. doi: 10.1016/j.talanta.2016.07.011
9. [9]
  A. Kumar, V. Santhanam, Anal. Chim. Acta1090 (2019) 106–113. doi: 10.1038/s41929-018-0218-y
10. [10]
  Y. Ai, P. Liang, Y. Wu, et al., Food Chem. 241 (2018) 427–433. doi: 10.1016/j.foodchem.2017.09.019
11. [11]
  Y.Y. Chao, Y.L. Chen, H.Y. Lin, et al., Anal. Chim. Acta1010 (2018) 44–53. doi: 10.1016/j.aca.2018.01.003
12. [12]
  H.M. Liu, H.D. Qiu, Chem. Eng. J. 393 (2020) 124691. doi: 10.1016/j.cej.2020.124691
13. [13]
  J. Chen, Z.J. Gong, W.Y. Tang, et al., TrAC Trends Anal. Chem. 134 (2021) 116135. doi: 10.1016/j.trac.2020.116135
14. [14]
  Y. Dong, S.W. Li, S.S. Hong, et al., Chin. Chem. Lett. 31 (2020) 635–642. doi: 10.1016/j.cclet.2019.08.021
15. [15]
  S. Rojas, P. Horcajada, Chem. Rev. 120, (2020), 8378–8415. doi: 10.1021/acs.chemrev.9b00797
16. [16]
  L.E. Kreno, K. Leong, O.K. Farha, et al., Chem. Rev. 112 (2012) 1105–1125. doi: 10.1021/cr200324t
17. [17]
  S. Zhang, X.B. Pei, H.L. Gao, et al., Chin. Chem. Lett. 31 (2020) 1060–1070. doi: 10.1016/j.cclet.2019.11.036
18. [18]
  F.H. Mu, B.L. Dai, W. Zhao, et al., Chin. Chem. Lett. 31 (2020) 1773–1781. doi: 10.1016/j.cclet.2019.12.015
19. [19]
  L.N. Li, Y.L. Chen, L. Yang, et al., Coord. Chem. Rev. 411 (2020) 213235. doi: 10.1016/j.ccr.2020.213235
20. [20]
  P.G. Qin, W.L. Zhu, L.Z. Han, et al., Microchim. Acta187 (2020) 367. doi: 10.1007/s00604-020-04326-3
21. [21]
  C.C. Pei, C. Liu, Y. Wang, et al., Angew. Chem. Int. Ed. 59 (2020) 10831–10835. doi: 10.1002/anie.202001135
22. [22]
  Y. Wang, Q. Ye, M.H. Yu, et al., Chin. Chem. Lett. 31 (2020) 1843–1846. doi: 10.1016/j.cclet.2020.02.054
23. [23]
  J.H. Cavka, S. Jakobsen, U. Olsbye, et al., J. Am. Chem. Soc. 130 (2008) 13850–13851. doi: 10.1021/ja8057953
24. [24]
  Z.Y. Gan, C.F. Huang, Y.F. Shen, et al., Chin. Chem. Lett. 31 (2020) 513–516. doi: 10.1016/j.cclet.2019.04.065
25. [25]
  Y.P. Sun, W.H. Ha, J. Chen, et al., TrAC Trends Anal. Chem. 84 (2016) 12–21. doi: 10.18088/ejbmr.2.2.2016.pp12-18
26. [26]
  G.C. Sun, F.Z. Zhang, Q.S. Xie, et al., Chin. Chem. Lett. 31 (2020) 1603–1607. doi: 10.1016/j.cclet.2019.10.018
27. [27]
  Y.X. Yang, P.G. Qin, X.T. Zhang, et al., Anal. Methods10 (2018) 322–329. doi: 10.1039/C7AY02515G
28. [28]
  Y.X. Yang, P.G. Qin, J. Zhang, et al., J. Chromatogr. A1570 (2018) 47–55. doi: 10.1016/j.chroma.2018.07.080
29. [29]
  J. Zhang, W.Q. Li, W.L. Zhu, et al., Chem. Comm. 55 (2019) 10019–10023. doi: 10.1039/c9cc04348a
30. [30]
  J. Zhang, W.Q. Li, W.L. Zhu, et al., Microchim. Acta186 (2019) 279. doi: 10.1007/s00604-019-3394-9
31. [31]
  F. Yang, W.Y. Li, B. Tang, J. Alloy. Compd. 733 (2018) 8–14. doi: 10.1016/j.jallcom.2017.10.129
32. [32]
  J.L. Tang, Y.B. Chen, M.H. Zhao, et al., J. Hazard. Mater. 413 (2021) 125278. doi: 10.1016/j.jhazmat.2021.125278
33. [33]
  M. Sarker, J.Y. Song, S.H. Jhung, Chem. Eng. J. 331 (2018) 124–131. doi: 10.1016/j.cej.2017.08.017
34. [34]
  H. Chen, X.J. Deng, G.S. Ding, Food Chem. 293 (2019) 340–347. doi: 10.1007/s10946-019-09809-0
35. [35]
  X.T. Zhang, J. Zhang, W.Q. Li, et al., Food Addit. Contam. A11 (2018) 2099–2110. doi: 10.1080/19440049.2018.1526415
36. [36]
  J.H. Chen, G.M. Zhou, H.Y. Qin, et al., Anal. Methods7 (2015), 6537–6544. doi: 10.1039/C5AY01105A
37. [37]
  X. Wang, N. Chen, Q. Han, et al., J. Sep. Sci. 38 (2015) 2167–2173. doi: 10.1002/jssc.201500014
38. [38]
  P.G. Qin, Y.X. Yang, W.Q. Li, et al., Anal. Methods11 (2019) 105–112. doi: 10.1039/c8ay02215a
1. [1]
  Jiayu Huang , Kuan Chang , Qi Liu , Yameng Xie , Zhijia Song , Zhiping Zheng , Qin Kuang . Fe-N-C nanostick derived from 1D Fe-ZIFs for Electrocatalytic oxygen reduction. Chinese Journal of Structural Chemistry, 2023, 42(10): 100097-100097. doi: 10.1016/j.cjsc.2023.100097
2. [2]
  Xiao-Hong Yi , Chong-Chen Wang . Metal-organic frameworks on 3D interconnected macroporous sponge foams for large-scale water decontamination: A mini review. Chinese Chemical Letters, 2024, 35(5): 109094-. doi: 10.1016/j.cclet.2023.109094
3. [3]
  Muhammad Riaz , Rakesh Kumar Gupta , Di Sun , Mohammad Azam , Ping Cui . Selective adsorption of organic dyes and iodine by a two-dimensional cobalt(II) metal-organic framework. Chinese Journal of Structural Chemistry, 2024, 43(12): 100427-100427. doi: 10.1016/j.cjsc.2024.100427
4. [4]
  Tengjia Ni , Xianbiao Hou , Huanlei Wang , Lei Chu , Shuixing Dai , Minghua Huang . Controllable defect engineering based on cobalt metal-organic framework for boosting oxygen evolution reaction. Chinese Journal of Structural Chemistry, 2024, 43(1): 100210-100210. doi: 10.1016/j.cjsc.2024.100210
5. [5]
  Mengyuan Li , Xitong Ren , Yanmei Gao , Mengyao Mu , Shiping Zhu , Shufang Tian , Minghua Lu . Constructing bifunctional magnetic porous poly(divinylbenzene) polymer for high-efficient removal and sensitive detection of bisphenols. Chinese Chemical Letters, 2024, 35(12): 109699-. doi: 10.1016/j.cclet.2024.109699
6. [6]
  Ze Liu , Xiaochen Zhang , Jinlong Luo , Yingjian Yu . Application of metal-organic frameworks to the anode interface in metal batteries. Chinese Chemical Letters, 2024, 35(11): 109500-. doi: 10.1016/j.cclet.2024.109500
7. [7]
  Longlong Geng , Huiling Liu , Wenfeng Zhou , Yong-Zheng Zhang , Hongliang Huang , Da-Shuai Zhang , Hui Hu , Chao Lv , Xiuling Zhang , Suijun Liu . Construction of metal-organic frameworks with unsaturated Cu sites for efficient and fast reduction of nitroaromatics: A combined experimental and theoretical study. Chinese Chemical Letters, 2024, 35(8): 109120-. doi: 10.1016/j.cclet.2023.109120
8. [8]
  Rui Wang , He Qi , Haijiao Zheng , Qiong Jia . Light/pH dual-responsive magnetic metal-organic frameworks composites for phosphorylated peptide enrichment. Chinese Chemical Letters, 2024, 35(7): 109215-. doi: 10.1016/j.cclet.2023.109215
9. [9]
  Fereshte Hassanzadeh-Afruzi , Mina Azizi , Iman Zare , Ehsan Nazarzadeh Zare , Anwarul Hasan , Siavash Iravani , Pooyan Makvandi , Yi Xu . Advanced metal-organic frameworks-polymer platforms for accelerated dermal wound healing. Chinese Chemical Letters, 2024, 35(11): 109564-. doi: 10.1016/j.cclet.2024.109564
10. [10]
  Yuan Zhang , Shenghao Gong , A.R. Mahammed Shaheer , Rong Cao , Tianfu Liu . Plasmon-enhanced photocatalytic oxidative coupling of amines in the air using a delicate Ag nanowire@NH₂-UiO-66 core-shell nanostructures. Chinese Chemical Letters, 2024, 35(4): 108587-. doi: 10.1016/j.cclet.2023.108587
11. [11]
  Jian Peng , Yue Jiang , Shuangyu Wu , Yanran Cheng , Jingyu Liang , Yixin Wang , Zhuo Li , Sijie Lin . A nonradical oxidation process initiated by Ti-peroxo complex showed high specificity toward the degradation of tetracycline antibiotics. Chinese Chemical Letters, 2024, 35(5): 108903-. doi: 10.1016/j.cclet.2023.108903
12. [12]
  Wenbiao Zhang , Bolong Yang , Zhonghua Xiang . Atomically dispersed Cu-based metal-organic framework directly for alkaline polymer electrolyte fuel cells. Chinese Chemical Letters, 2025, 36(2): 109630-. doi: 10.1016/j.cclet.2024.109630
13. [13]
  Xudong Zhao , Yuxuan Wang , Xinxin Gao , Xinli Gao , Meihua Wang , Hongliang Huang , Baosheng Liu . Anchoring thiol-rich traps in 1D channel wall of metal-organic framework for efficient removal of mercury ions. Chinese Chemical Letters, 2025, 36(2): 109901-. doi: 10.1016/j.cclet.2024.109901
14. [14]
  Zhefei Hu , Jingwen Liao , Jiawen Zhou , Lulu Zhao , Yanjuan Liu , Yuefei Zhang , Wei Chen , Sheng Tang . A new green approach to synthesizing MIP-202@porous silica microspheres for positional isomer/enantiomer/hydrophilic separation. Chinese Chemical Letters, 2025, 36(1): 109985-. doi: 10.1016/j.cclet.2024.109985
15. [15]
  Zhi Wang , Lingpeng Yan , Yelin Hao , Jingxia Zheng , Yongzhen Yang , Xuguang Liu . Highly efficient and photothermally stable CDs@ZIF-8 for laser illumination. Chinese Chemical Letters, 2024, 35(10): 109430-. doi: 10.1016/j.cclet.2023.109430
16. [16]
  Hao Wang , Meng-Qi Pan , Ya-Fei Wang , Chao Chen , Jian Xu , Yuan-Yuan Gao , Chuan-Song Qi , Wei Li , Xian-He Bu . Post-synthetic modifications of MOFs by different bolt ligands for controllable release of cargoes. Chinese Chemical Letters, 2024, 35(10): 109581-. doi: 10.1016/j.cclet.2024.109581
17. [17]
  Yan-Kai Zhang , Yong-Zheng Zhang , Chun-Xiao Jia , Fang Wang , Xiuling Zhang , Yuhang Wu , Zhongmin Liu , Hui Hu , Da-Shuai Zhang , Longlong Geng , Jing Xu , Hongliang Huang . A stable Zn-MOF with anthracene-based linker for Cr(VI) photocatalytic reduction under sunlight irradiation. Chinese Chemical Letters, 2024, 35(12): 109756-. doi: 10.1016/j.cclet.2024.109756
18. [18]
  Ruowen Liang , Chao Zhang , Guiyang Yan . Enhancing CO2 cycloaddition through ligand functionalization: A case study of UiO-66 metal-organic frameworks. Chinese Journal of Structural Chemistry, 2024, 43(2): 100211-100211. doi: 10.1016/j.cjsc.2023.100211
19. [19]
  Benjian Xin , Rui Wang , Lili Liu , Zhiqiang Niu . Metal-organic framework derived MnO@C/CNTs composite for high-rate lithium-based semi-solid flow batteries. Chinese Journal of Structural Chemistry, 2023, 42(11): 100116-100116. doi: 10.1016/j.cjsc.2023.100116
20. [20]
  Ruikui YAN , Xiaoli CHEN , Miao CAI , Jing REN , Huali CUI , Hua YANG , Jijiang WANG . Design, synthesis, and fluorescence sensing performance of highly sensitive and multi-response lanthanide metal-organic frameworks. Chinese Journal of Inorganic Chemistry, 2024, 40(4): 834-848. doi: 10.11862/CJIC.20230301

Get Citation

PDF

XML

Metrics

PDF Downloads(7)
Abstract views(882)
HTML views(63)

通讯作者: 陈斌, bchen63@163.com

1.
沈阳化工大学材料科学与工程学院沈阳 110142

Facile preparation of nano-g-C3N4/UiO-66-NH2 composite as sorbent for high-efficient extraction and preconcentration of food colorants prior to HPLC analysis

Metrics

通讯作者: 陈斌, bchen63@163.com

Facile preparation of nano-g-C₃N₄/UiO-66-NH₂ composite as sorbent for high-efficient extraction and preconcentration of food colorants prior to HPLC analysis