Citation: Zhiwen Jiang, Yusong Wang, Guoqing Xu, Zhuoni Jiang, Zhiqing Ge, Mozhen Wang, Xuewu Ge. Flexible, high sensitive and radiation-resistant pressure-sensing hydrogel[J]. Chinese Chemical Letters, ;2022, 33(2): 1011-1016. doi: 10.1016/j.cclet.2021.06.043 shu

Flexible, high sensitive and radiation-resistant pressure-sensing hydrogel

Zhiwen Jiang ^a ,
Yusong Wang ^b ,
Guoqing Xu ^a ,
Zhuoni Jiang ^a ,
Zhiqing Ge ^a ,
Mozhen Wang ^{a, *,} ,
Xuewu Ge ^{a, *,}

a.
CAS Key Laboratory of Soft Matter Chemistry, Department of Polymer Science and Engineering, University of Science and Technology of China, Hefei 230026, China
b.
Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei 230026, China

pstwmz@ustc.edu.cn

xwge@ustc.edu.cn

Received Date: 14 April 2021
Revised Date: 8 June 2021
Accepted Date: 15 June 2021
Available Online: 22 June 2021

Figures(5)

Excellent radiation resistance is a prerequisite for pressure-sensitive hydrogels to be used in high-energy radiation environments. In this work, tannic acid-modified boron nitride nanosheet (BNNS-TA) is first prepared as the radiation-resistant additive by a facile one-step ball milling of hexagonal boron nitride and tannic acid. Then, polyacrylamide (PAAm)-based pressure-sensitive hydrogel doped with BNNS-TA and Fe³⁺ ions is fabricated. The ternary BNNS-TA/Fe³⁺/PAAm hydrogel exhibits excellent compressive strength (at least four times the compressive strength of unfilled pure PAAm hydrogel), pressure-sensitive performance (gauge factor is up to 1.4), and performance recovery due to the combination of multiple intermolecular interactions, such as covalent crosslinking, hydrogen bonds, and ion coordination interactions. The BNNS-TA/Fe³⁺/PAAm hydrogel can be made as a pressure sensor installed in the control circuit or attached on the human body to detect human activities accurately. More importantly, the compressive strength and the pressure-sensitive performance of the BNNS-TA/Fe³⁺/PAAm hydrogel can be maintained after the hydrogel is irradiated by ⁶⁰Co gamma-ray at an absorbed dose of 15 kGy. As a comparison, the compressive strength of the unfilled PAAm hydrogel is only a quarter of that before irradiation. This work not only reveals a facile method to achieve the preparation of chemically modified BNNS as a promising radiation-resistant additive but also provides a novel strategy for the development of pressure-sensitive hydrogel devices in radiation environments.
- Pressure-sensitive hydrogel,
- Polyacrylamide,
- Radiation resistance,
- Boron nitride nanosheet,
- Tannic acid,
- Motion detection
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