Citation: Dongli Guo, Shijie You, Fang Li, Yanbiao Liu. Engineering carbon nanocatalysts towards efficient degradation of emerging organic contaminants via persulfate activation: A review[J]. Chinese Chemical Letters, ;2022, 33(1): 1-10. doi: 10.1016/j.cclet.2021.06.027 shu

Engineering carbon nanocatalysts towards efficient degradation of emerging organic contaminants via persulfate activation: A review

Dongli Guo ^b ,
Shijie You ^{a, *,} ,
Fang Li ^b ,
Yanbiao Liu ^{b, *,}

a.
State Key Laboratory of Urban Water Resource and Environment, School of Environment, Harbin Institute of Technology, Harbin 150090, China
b.
Textile Pollution Controlling Engineering Center of Ministry of Environmental Protection, College of Environmental Science and Engineering, Donghua University, Shanghai 201620, China

yanbiaoliu@dhu.edu.cn

ashen8212@gmail.com

Received Date: 30 March 2021
Revised Date: 21 April 2021
Accepted Date: 10 June 2021
Available Online: 17 June 2021

Figures(6)

The engineering of carbon nanocatalysts for the persulfate activated elimination of emerging organic contaminants (EOCs) demonstrates promising potential compared with metal-based counterparts due to their unique advantage of high stability and low toxicity. The early reviews introduced the theoretical background of persulfate activation together with a detailed summary of different mechanisms responsible for degradation of EOCs. To further unify the state of knowledge, identify the research gaps, and prompt new research in this area, we present a thorough review on current trends in research on metal-free carbon nanocatalysts (e.g., 0D nanodiamond, 1D carbon nanotubes and carbon nanofibers, 2D graphene and graphitic carbon nitride, and 3D carbon nanocatalysts), with emphasis on their applications in persulfate activation and EOCs decontamination. We also discuss the current challenges and future perspectives in practically relevant applications. Last, we highlight that the development of sustainable carbon nanocatalysts/persulfate systems lies at the interface of multiple disciplines, which calls for future in-depth interdisciplinary collaborations.
- Carbon nanocatalysts,
- Persulfate activation,
- Advanced oxidation processes,
- Emerging organic contaminants,
- Water purification
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沈阳化工大学材料科学与工程学院沈阳 110142