Citation: Deling Yuan, Chen Zhang, Shoufeng Tang, Zetao Wang, Qina Sun, Xiaoyu Zhang, Tifeng Jiao, Qingrui Zhang. Ferric ion-ascorbic acid complex catalyzed calcium peroxide for organic wastewater treatment: Optimized by response surface method[J]. Chinese Chemical Letters, ;2021, 32(11): 3387-3392. doi: 10.1016/j.cclet.2021.04.050 shu

Ferric ion-ascorbic acid complex catalyzed calcium peroxide for organic wastewater treatment: Optimized by response surface method

Deling Yuan ^{a, b} ,
Chen Zhang ^a ,
Shoufeng Tang ^{a, b, *,} ,
Zetao Wang ^a ,
Qina Sun ^a ,
Xiaoyu Zhang ^a ,
Tifeng Jiao ^{a, b, *,} ,
Qingrui Zhang ^{a, b}

a.
Hebei Key Laboratory of Heavy Metal Deep-Remediation in Water and Resource Reuse, Hebei Key Laboratory of Applied Chemistry, School of Environmental and Chemical Engineering, Yanshan University, Qinhuangdao 066004, China
b.
State Key Laboratory of Metastable Materials Science and Technology, Yanshan University, Qinhuangdao 066004, China

tangshf@ysu.edu.cn

tfjiao@ysu.edu.cn

Received Date: 30 January 2021
Revised Date: 15 April 2021
Accepted Date: 27 April 2021
Available Online: 4 May 2021

Figures(4)

Hydrogen peroxide (H₂O₂) disproportionation, iron precipitation, and narrow pH range are the drawbacks of traditional Fenton process. To surmount these barriers, we proposed a ferric ion (Fe³⁺)-ascorbic acid (AA) complex catalyzed calcium peroxide (CaO₂) Fenton-like system to remove organic dyes in water. This collaborative Fe³⁺/AA/CaO₂ system presented an obvious improvement in the methyl orange (MO) decolorization, and also effectively eliminated other dyes. Response surface method was employed to optimize the running parameters for this coupling process. Under the optimized arguments (2.76 mmol/L Fe³⁺, 0.68 mmol/L AA, and 4 mmol/L CaO₂), the MO removal achieved 98.90% after 15 min at pH 6.50, which was close to the computed outcome of 99.30%. Furthermore, this Fenton-like system could perform well in a wide range of pH (3-11), and enhance the H₂O₂ decomposition and Fe ions recycle. The scavenger experiment result indicated that hydroxyl radical, superoxide anion free radical, and singlet oxygen were acted on the dye elimination. Moreover, electron spin resonance analysis corroborated that the existences of these active species in the Fe³⁺/AA/CaO₂ system. This study could advance the development of Fenton-like technique in organic effluent disposal.
- Ferric ion,
- Ascorbic acid,
- Calcium peroxide,
- Response surface method,
- Dye removal
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