Citation: Hongfei Wang, Yijun Zhong, Jiqiang Ning, Yong Hu. Recent advances in the synthesis of non-carbon two-dimensional electrode materials for the aqueous electrolyte-based supercapacitors[J]. Chinese Chemical Letters, ;2021, 32(12): 3733-3752. doi: 10.1016/j.cclet.2021.04.025 shu

Recent advances in the synthesis of non-carbon two-dimensional electrode materials for the aqueous electrolyte-based supercapacitors

Hongfei Wang ^{a, b} ,
Yijun Zhong ^a ,
Jiqiang Ning ^c ,
Yong Hu ^{a, *,}

a.
Key Laboratory of the Ministry of Education for Advanced Catalysis Materials, Department of Chemistry, Zhejiang Normal University, Jinhua 321004, China
b.
Department of Chemical Physics, University of Science and Technology of China, Hefei 230026, China
c.
Vacuum Interconnected Nanotech Workstation, Suzhou Institute of Nano-Tech and Nano-Bionics, Chinese Academy of Sciences, Suzhou 215123, China

Author Bio: Hongfei Wang received his Ph.D. degree from University of Science and Technology of China in 2021, and now he joined Zhejiang Normal University as a lecturer. His work focuses on the preparation of advanced electrode materials and hydrogel electrolytes in supercapacitors, as well as the synthesis of catalysts towards methanol electrooxidation reaction
Yijun Zhong is a Full Professor at the College of Chemistry and Life Science, Zhejiang Normal University (ZJNU), China. He joined ZJNU in 1983 and is a visiting fellow at Institution of Catalysis, Zhejiang University for two years. He received his Ph.D. degree in Industrial Catalysis from Zhejiang University of Technology, China in 2008. His research interests include the design and application of inorganic nanostructures for industrial catalysis and energy conversion and storage
Jiqiang Ning received his B.S. degree in 2000 and M.E. degree in 2003, both from the University of Science and Technology of China (USTC), and his Ph.D. degree in 2007 from the University of Hong Kong (HKU) where he then worked as a postdoctoral researcher in the lab of laser spectroscopy at the Physics Department. He is currently a professor at Suzhou Institute of Nano-tech and Nano-Bionics (SINANO), Chinese Academy of Sciences (CAS), and his current research is focused on optical spectroscopic studies on non-linear optical phenomena, electronic behaviors and defect states in semiconductors and their nanostructures
Yong Hu obtained his Ph.D. degree in Inorganic Chemistry in 2006 at University of Science and Technology of China (USTC). He then worked as a research fellow at Nanyang Technological University (NTU). Stating from 2008, he is a full professor at the College of Chemistry and Life Science, Zhejiang Normal University (ZJNU), China. His current research interests are focused on the design and synthesis of nanomaterials for energy and environmental applications

yonghu@zjnu.edu.cn

Received Date: 25 March 2021
Revised Date: 12 April 2021
Accepted Date: 13 April 2021
Available Online: 24 April 2021

Figures(12)

Supercapacitors (SCs) with high power density and long cycling span life are demanding energy storage devices that will be an attractive power solution to modern electronic and electrical applications. Numerous theoretical and experimental works have been devoted to exploring various possibilities to increase the functionality and the specific capacitance of electrodes for SCs. Non-carbon two-dimensional (2D) materials have been considered as encouraging electrode candidates for their chemical and physical advantages such as tunable surface chemistry, high electronic conductivity, large mechanical strength, more active sites, and dual non-faradaic and faradaic electrochemical performances. Besides, these 2D materials also play particular roles in constructing highway channels for fast ion diffusion. This concise review summarizes cutting-edge progress of some representative 2D non-carbon materials for the aqueous electrolyte-based SCs, including transition metal oxides (TMOs), transition metal hydroxides (TMHs), transition metal chalcogenides (TMCs), MXenes, metal-organic frameworks (MOFs) and some emerging materials. Different synthetic methods, effective structural designs and corresponding electrochemical performances are reviewed in detail. And we finally present a detailed discussion of the current intractable challenges and technical bottlenecks, and highlight future directions and opportunities for the development of next-generation high-performance energy storage devices.
- Supercapacitors,
- 2D non-carbon materials,
- Aqueous electrolyte,
- High power density,
- Long cycling span life
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