Citation: Zelin Cai, Zilin Peng, Xinlong Liu, Rui Sun, Zhaoxia Qin, Haosen Fan, Yufei Zhang. Improving Na⁺ transport kinetics and Na⁺ storage of hierarchical rhenium-nickel sulfide (ReS₂@NiS₂) hollow architecture by assembling layered 2D-3D heterostructures[J]. Chinese Chemical Letters, ;2021, 32(11): 3607-3612. doi: 10.1016/j.cclet.2021.04.011 shu

Improving Na⁺ transport kinetics and Na⁺ storage of hierarchical rhenium-nickel sulfide (ReS₂@NiS₂) hollow architecture by assembling layered 2D-3D heterostructures

Zelin Cai ^a ,
Zilin Peng ^a ,
Xinlong Liu ^a ,
Rui Sun ^a ,
Zhaoxia Qin ^a ,
Haosen Fan ^{a, *,} ,
Yufei Zhang ^{b, *,}

a.
School of Chemistry and Chemical Engineering, Guangzhou University, Guangzhou 510006, China
b.
School of Chemical Engineering and Light Industry, Guangdong University of Technology, Guangzhou 510006, China

hsfan@gzhu.edu.cn

yfzhang@gdut.edu.cn

Received Date: 27 February 2021
Revised Date: 30 March 2021
Accepted Date: 5 April 2021
Available Online: 7 April 2021

Figures(5)

Mixed metal sulfides have been widely used as anode material of sodium-ion batteries (SIBs) because of their excellent conductivity and sodium ion storage performance. Herein, ReS₂@NiS₂ heterostructures have been triumphantly designed and prepared through anchoring ReS₂ nanosheet arrays on the surface of NiS₂ hollow nanosphere. Specifically, the carbon nanospheres was used as hard template to synthesize NiS₂ hollow spheres as the substrate and then the ultrathin two-dimensional ReS₂ nanosheet arrays were uniformly grown on the surface of NiS₂. The internal hollow property provides sufficient space to relieve the volume expansion, and the outer two-dimensional nanosheet realizes the rapid electron transport and insertion/extraction of Na⁺. Owing to the great improvement of the transport kinetics of Na⁺, NiS₂@ReS₂ heterostructure electrode can achieve a high specific capacity of 400 mAh/g at the high current density of 1 A/g and still maintain a stable cycle stability even after 220 cycles. This hard template method not only paves a new way for the design and construct binary metal sulfide heterostructure electrode materials with outstanding electrochemical performance for Na⁺ batteries but also open up the potential applications of anode materials of SIBs.
- Nanosheet arrays,
- Diffusion kinetics,
- NiS₂@ReS₂,
- Sodium storage,
- Heterostructure
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通讯作者: 陈斌, bchen63@163.com

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沈阳化工大学材料科学与工程学院沈阳 110142

Improving Na+ transport kinetics and Na+ storage of hierarchical rhenium-nickel sulfide (ReS2@NiS2) hollow architecture by assembling layered 2D-3D heterostructures

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通讯作者: 陈斌, bchen63@163.com

Improving Na⁺ transport kinetics and Na⁺ storage of hierarchical rhenium-nickel sulfide (ReS₂@NiS₂) hollow architecture by assembling layered 2D-3D heterostructures