Citation: Yanxi Chen, Shenyu Lan, Mingshan Zhu. Construction of piezoelectric BaTiO₃/MoS₂ heterojunction for boosting piezo-activation of peroxymonosulfate[J]. Chinese Chemical Letters, ;2021, 32(6): 2052-2056. doi: 10.1016/j.cclet.2020.11.016 shu

Construction of piezoelectric BaTiO₃/MoS₂ heterojunction for boosting piezo-activation of peroxymonosulfate

Guangdong Key Laboratory of Environmental Pollution and Health, School of Environment, Jinan University, Guangzho, 511443, China

zhumingshan@jnu.edu.cn

Received Date: 10 October 2020
Revised Date: 1 November 2020
Accepted Date: 9 November 2020
Available Online: 11 November 2020

Figures(4)

The rapid recombination of charge carriers in piezoelectric materials has always been the problem that limits their piezoelectric performance for removal of organic pollutants in water. Herein, we construct a piezoelectric BaTiO₃/MoS₂ (BTO/MS) that follows a type Ⅱ heterojunction charge transfer system to inhibit the recombination of electron-hole (e^‒-h⁺) pairs, which is beneficial to the activation of peroxymonosulfate (PMS) for the removal of antibiotic ornidazole (ORZ) pollutants. The optimal ratio of BTO/MS for ORZ degradation under the piezo/PMS process is 13.9, 3.6, 62.1 and 2.0 times higher than that of the BTO/piezo, MS/piezo, (BTO/MS)/PMS and (BTO/MS)/piezo processes, respectively. The high efficiency charge separation in the piezoelectric heterojunction of BTO/MS promotes the activation of PMS, resulting in the synergy of pizeocatalysis and PMS oxidation during the process of ORZ degradation. This study provides an idea for enhancing piezo-activation of PMS by constructing heterojunctions in piezoelectric materials.
- Piezoelectricity,
- Peroxymonosulfate,
- BaTiO₃/MoS₂ Heterojunction,
- Ornidazole degradation
1. [1]
  W. Ahmad, A. Singh, K.K. Jaiswal, P. Gupta, J. Inorg. Organomet. P. 31(2021) 614-623. doi: 10.1007/s10904-020-01703-6
2. [2]
  R. Tan, Z. Lv, J. Tang, et al., Sci. Rep. 9(2019) 10891. doi: 10.1038/s41598-018-37645-w
3. [3]
  D. Li, W. Shi, Chinese J. Catal. 37(2016) 792-799. doi: 10.1016/S1872-2067(15)61054-3
4. [4]
  T. Bergan, Scand. J. Infect. Dis. 46(1985) 64-71.
5. [5]
  R. Yin, Y. Chen, S. He, et al., J. Hazard. Mater. 388(2020) 121996. doi: 10.1016/j.jhazmat.2019.121996
6. [6]
  C. Qi, X. Liu, J. Ma, et al., Chemosphere 151(2016) 280-288. doi: 10.1016/j.chemosphere.2016.02.089
7. [7]
  Q. Chen, L. Chen, J. Qi, et al., Chin. Chem. Lett. 30(2019) 1214-1218. doi: 10.1016/j.cclet.2019.03.002
8. [8]
  S. Xiao, M. Cheng, H. Zhong, et al., Chem. Eng. J. 384(2020) 123265. doi: 10.1016/j.cej.2019.123265
9. [9]
  J. Wang, S. Wang, Chem. Eng. J. 334(2018) 1502-1517. doi: 10.1016/j.cej.2017.11.059
10. [10]
  M. Zhang, J. He, Y. Chen, et al., Chin. Chem. Lett. 31(2020) 2721-2724. doi: 10.1016/j.cclet.2020.05.001
11. [11]
  S. Nimai, H. Zhang, Z. Wu, N. Li, B. Lai, Chin. Chem. Lett. 31(2020) 2657-2660. doi: 10.1016/j.cclet.2020.08.008
12. [12]
  H. Zhang, Q. Ji, L. Lai, G. Yao, B. Lai, Chin. Chem. Lett. 30(2019) 1129-1132. doi: 10.1016/j.cclet.2019.01.025
13. [13]
  S. Yang, P. Wang, X. Yang, et al., J. Hazard. Mater. 179(2010) 552-558. doi: 10.1016/j.jhazmat.2010.03.039
14. [14]
  S.Y. Oh, H.W. Kim, J.M. Park, H.S. Park, C. Yoon, J. Hazard. Mater. 168(2009) 346-351. doi: 10.1016/j.jhazmat.2009.02.065
15. [15]
  G. Zhen, X. Lu, L. Su, et al., Water Res. 134(2018) 101-114. doi: 10.1016/j.watres.2018.01.072
16. [16]
  S. Lan, J. Feng, Y. Xiong, et al., Environ. Sci. Technol. 51(2017) 6560-6569. doi: 10.1021/acs.est.6b06426
17. [17]
  Y. Chen, X. Deng, J. Wen, J. Zhu, Z. Bian, Appl. Catal. B: Environ. 258(2019) 118024. doi: 10.1016/j.apcatb.2019.118024
18. [18]
  Y. Feng, L. Ling, Y. Wang, et al., Nano Energy 40(2017) 481-486. doi: 10.1016/j.nanoen.2017.08.058
19. [19]
  Z.L. Wang, J. Song, Science 312(2006) 242-246. doi: 10.1126/science.1124005
20. [20]
  Z.L. Wang, Adv. Mater. 24(2012) 4632-4646. doi: 10.1002/adma.201104365
21. [21]
  L. Pan, S. Sun, Y. Chen, et al., Adv. Energy Mater. 10(2020) 2000214. doi: 10.1002/aenm.202000214
22. [22]
  H. Huang, S. Tu, C. Zeng, et al., Angew. Chem. Int. Edit. 56(2017) 11860-11864. doi: 10.1002/anie.201706549
23. [23]
  S. Lan, Y. Chen, L. Zeng, et al., J. Hazard. Mater. 393(2020) 122448. doi: 10.1016/j.jhazmat.2020.122448
24. [24]
  S. Lan, X. Zeng, R.A. Rather, I.M.C. Lo, Environ. Sci. Nano 6(2019) 554-564. doi: 10.1039/C8EN01192C
25. [25]
  Y. Feng, H. Li, L. Ling, et al., Environ Sci. Technol. 52(2018) 7842-7848. doi: 10.1021/acs.est.8b00946
26. [26]
  S. Tu, Y. Guo, Y. Zhang, et al., Adv. Funct. Mater. 30(2020) 2005158. doi: 10.1002/adfm.202005158
27. [27]
  P. Wang, X. Li, S. Fan, et al., Appl. Catal. B: Environ. 279(2020) 119340. doi: 10.1016/j.apcatb.2020.119340
28. [28]
  X. Liu, L. Xiao, Y. Zhang, H. Sun, J. Materiomics 6(2020) 256-262. doi: 10.1016/j.jmat.2020.03.004
29. [29]
  J. Wu, N. Qin, D. Bao, Nano Energy 45(2018) 44-51. doi: 10.1016/j.nanoen.2017.12.034
30. [30]
  S. Xu, L. Guo, Q. Sun, Z.L. Wang, Adv. Funct. Mater. 29(2019) 1808737. doi: 10.1002/adfm.201808737
31. [31]
  W. Lv, L. Kong, S. Lan, et al., J. Chem. Technol. Biot. 92(2017) 152-156. doi: 10.1002/jctb.4981
32. [32]
  X. Zhou, S. Wu, C. Li, et al., Nano Energy 66(2019) 104127. doi: 10.1016/j.nanoen.2019.104127
33. [33]
  X. Zhao, Y. Lei, P. Fang, et al., Nano Energy 66(2019) 104168. doi: 10.1016/j.nanoen.2019.104168
34. [34]
  M. Dai, W. Zheng, X. Zhang, et al., Nano lett. 20(2019) 201-207.
35. [35]
  H. Zhang, J. He, C. Zhai, M. Zhu, Chin. Chem. Lett. 30(2019) 2338-2342. doi: 10.1016/j.cclet.2019.07.021
36. [36]
  Q. Wang, Y. Qiu, D. Yang, et al., Appl. Phys. Lett. 113(2018) 053901. doi: 10.1063/1.5035309
37. [37]
  J. Wang, Q. Zhang, F. Deng, X. Luo, D.D. Dionysiou, Chem. Eng. J. 379(2020) 122264. doi: 10.1016/j.cej.2019.122264
38. [38]
  C. Morell, A. Grand, A. Toro-Labbe, J. Phy. Chem. A 109(2005) 205-212. doi: 10.1021/jp046577a
39. [39]
  J. Zhao, B. Yao, Q. He, T. Zhang, J. Hazard. Mater. 229(2012) 151-158.
40. [40]
  R. Changotra, J.P. Guin, S.A. Khader, A. Dhir, J. Environ. Chem. Eng. 8(2020) 104423. doi: 10.1016/j.jece.2020.104423
1. [1]
  Mengmeng Ao , Jian Wei , Chuan-Shu He , Heng Zhang , Zhaokun Xiong , Yonghui Song , Bo Lai . Insight into the activation of peroxymonosulfate by N-doped copper-based carbon for efficient degradation of organic pollutants: Synergy of nonradicals. Chinese Chemical Letters, 2025, 36(1): 109882-. doi: 10.1016/j.cclet.2024.109882
2. [2]
  Yun-Xin Huang , Lin-Qian Yu , Ke-Yu Chen , Hao Wang , Shou-Yan Zhao , Bao-Cheng Huang , Ren-Cun Jin . Biochar with self-doped N to activate peroxymonosulfate for bisphenol-A degradation via electron transfer mechanism: The active edge graphitic N site. Chinese Chemical Letters, 2024, 35(9): 109437-. doi: 10.1016/j.cclet.2023.109437
3. [3]
  Dong Cheng , Youyou Feng , Bingxi Feng , Ke Wang , Guoxin Song , Gen Wang , Xiaoli Cheng , Yonghui Deng , Jing Wei . Polyphenol-mediated interfacial deposition strategy for supported manganese oxide catalysts with excellent pollutant degradation performance. Chinese Chemical Letters, 2024, 35(5): 108623-. doi: 10.1016/j.cclet.2023.108623
4. [4]
  Ming-Zhen Li , Yang Zhang , Kun Li , Ya-Nan Shang , Yi-Zhen Zhang , Yu-Jiao Kan , Zhi-Yang Jiao , Yu-Yuan Han , Xiao-Qiang Cao . In situ regeneration of catalyst for Fenton-like degradation by photogenerated electron transportation: Characterization, performance and mechanism comparison. Chinese Chemical Letters, 2025, 36(1): 109885-. doi: 10.1016/j.cclet.2024.109885
5. [5]
  Yu Yao , Jinqiang Zhang , Yantao Wang , Kunsheng Hu , Yangyang Yang , Zhongshuai Zhu , Shuang Zhong , Huayang Zhang , Shaobin Wang , Xiaoguang Duan . Nitrogen-rich carbon for catalytic activation of peroxymonosulfate towards green synthesis. Chinese Chemical Letters, 2024, 35(11): 109633-. doi: 10.1016/j.cclet.2024.109633
6. [6]
  Yinyin Xu , Yuanyuan Li , Jingbo Feng , Chen Wang , Yan Zhang , Yukun Wang , Xiuwen Cheng . Covalent organic frameworks doped with manganese-metal organic framework for peroxymonosulfate activation. Chinese Chemical Letters, 2024, 35(4): 108838-. doi: 10.1016/j.cclet.2023.108838
7. [7]
  Ying-Yu Zhang , Jia-Qi Luo , Yan Han , Wan-Ying Zhang , Yi Zhang , Hai-Feng Lu , Da-Wei Fu . Bistable switch molecule DPACdCl₄ showing four physical channels and high phase transition temperature. Chinese Chemical Letters, 2025, 36(1): 109530-. doi: 10.1016/j.cclet.2024.109530
8. [8]
  Kexin Yin , Jingren Yang , Yanwei Li , Qian Li , Xing Xu . Metal-free diatomaceous carbon-based catalyst for ultrafast and anti-interference Fenton-like oxidation. Chinese Chemical Letters, 2024, 35(12): 109847-. doi: 10.1016/j.cclet.2024.109847
9. [9]
  Cunjun Li , Wencong Liu , Xianlei Chen , Liang Li , Shenyu Lan , Mingshan Zhu . Adsorption and activation of peroxymonosulfate on BiOCl for carbamazepine degradation: The role of piezoelectric effect. Chinese Chemical Letters, 2024, 35(10): 109652-. doi: 10.1016/j.cclet.2024.109652
10. [10]
  Ruiying Liu , Li Zhao , Baishan Liu , Jiayuan Yu , Yujie Wang , Wanqiang Yu , Di Xin , Chaoqiong Fang , Xuchuan Jiang , Riming Hu , Hong Liu , Weijia Zhou . Modulating pollutant adsorption and peroxymonosulfate activation sites on Co3O4@N,O doped-carbon shell for boosting catalytic degradation activity. Chinese Journal of Structural Chemistry, 2024, 43(8): 100332-100332. doi: 10.1016/j.cjsc.2023.100332
11. [11]
  Ruonan Guo , Heng Zhang , Changsheng Guo , Ningqing Lv , Beidou Xi , Jian Xu . Degradation of neonicotinoids with different molecular structures in heterogeneous peroxymonosulfate activation system through different oxidation pathways. Chinese Chemical Letters, 2024, 35(9): 109413-. doi: 10.1016/j.cclet.2023.109413
12. [12]
  Zhiwen HU , Weixia DONG , Qifu BAO , Ping LI . Low-temperature synthesis of tetragonal BaTiO₃ for piezocatalysis. Chinese Journal of Inorganic Chemistry, 2024, 40(5): 857-866. doi: 10.11862/CJIC.20230462
13. [13]
  Zhiwen HU , Ping LI , Yulong YANG , Weixia DONG , Qifu BAO . Morphology effects on the piezocatalytic performance of BaTiO₃. Chinese Journal of Inorganic Chemistry, 2025, 41(2): 339-348. doi: 10.11862/CJIC.20240172
14. [14]
  Xingmin Chen , Yunyun Wu , Yao Tang , Peishen Li , Shuai Gao , Qiang Wang , Wen Liu , Sihui Zhan . Construction of Z-scheme Cu-CeO₂/BiOBr heterojunction for enhanced photocatalytic degradation of sulfathiazole. Chinese Chemical Letters, 2024, 35(7): 109245-. doi: 10.1016/j.cclet.2023.109245
15. [15]
  Juan WANG , Zhongqiu WANG , Qin SHANG , Guohong WANG , Jinmao LI . NiS and Pt as dual co-catalysts for the enhanced photocatalytic H₂ production activity of BaTiO₃ nanofibers. Chinese Journal of Inorganic Chemistry, 2024, 40(9): 1719-1730. doi: 10.11862/CJIC.20240102
16. [16]
  Shuqi Yu , Yu Yang , Keisuke Kuroda , Jian Pu , Rui Guo , Li-An Hou . Selective removal of Cr(Ⅵ) using polyvinylpyrrolidone and polyacrylamide co-modified MoS₂ composites by adsorption combined with reduction. Chinese Chemical Letters, 2024, 35(6): 109130-. doi: 10.1016/j.cclet.2023.109130
17. [17]
  Pingping HAO , Fangfang LI , Yawen WANG , Houfen LI , Xiao ZHANG , Rui LI , Lei WANG , Jianxin LIU . Hydrogen production performance of the non-platinum-based MoS₂/CuS cathode in microbial electrolytic cells. Chinese Journal of Inorganic Chemistry, 2024, 40(9): 1811-1824. doi: 10.11862/CJIC.20240054
18. [18]
  Junan Pan , Xinyi Liu , Huachao Ji , Yanwei Zhu , Yanling Zhuang , Kang Chen , Ning Sun , Yongqi Liu , Yunchao Lei , Kun Wang , Bao Zang , Longlu Wang . The strategies to improve TMDs represented by MoS₂ electrocatalytic oxygen evolution reaction. Chinese Chemical Letters, 2024, 35(11): 109515-. doi: 10.1016/j.cclet.2024.109515
19. [19]
  Chunyan Yang , Qiuyu Rong , Fengyin Shi , Menghan Cao , Guie Li , Yanjun Xin , Wen Zhang , Guangshan Zhang . Rationally designed S-scheme heterojunction of BiOCl/g-C₃N₄ for photodegradation of sulfamerazine: Mechanism insights, degradation pathways and DFT calculation. Chinese Chemical Letters, 2024, 35(12): 109767-. doi: 10.1016/j.cclet.2024.109767
20. [20]
  Fei ZHOU , Xiaolin JIA . Co₃O₄/TiO₂ composite photocatalyst: Preparation and synergistic degradation performance of toluene. Chinese Journal of Inorganic Chemistry, 2024, 40(11): 2232-2240. doi: 10.11862/CJIC.20240236

Get Citation

PDF

XML

Metrics

PDF Downloads(10)
Abstract views(835)
HTML views(67)

通讯作者: 陈斌, bchen63@163.com

1.
沈阳化工大学材料科学与工程学院沈阳 110142

Construction of piezoelectric BaTiO3/MoS2 heterojunction for boosting piezo-activation of peroxymonosulfate

Metrics

通讯作者: 陈斌, bchen63@163.com

Construction of piezoelectric BaTiO₃/MoS₂ heterojunction for boosting piezo-activation of peroxymonosulfate