Citation: Hongjun Dong, Ning Song, Ming Yan, Huihui Wu, Haibo Zhang, Changchang Ma, Yun Wang. Fabrication of HRP/Bi₂WO₆ photoenzyme-coupled artificial catalytic system for efficiently degrading bisphenol A[J]. Chinese Chemical Letters, ;2021, 32(6): 2047-2051. doi: 10.1016/j.cclet.2020.11.015 shu

Fabrication of HRP/Bi₂WO₆ photoenzyme-coupled artificial catalytic system for efficiently degrading bisphenol A

Hongjun Dong ^a ,
Ning Song ^a ,
Ming Yan ^a ,
Huihui Wu ^a ,
Haibo Zhang ^a ,
Changchang Ma ^b ,
Yun Wang ^{a, *,}

a.
Advanced Chemical Engineering Laboratory of Green Materials and Energy of Jiangsu Province, Institute of Green Chemistry and Chemical Technology, School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang 212013, China
b.
Department of Chemistry, Dongguk University, Seoul 04620, Republic of Korea

yunwang@ujs.edu.cn

Received Date: 14 September 2020
Revised Date: 15 October 2020
Accepted Date: 9 November 2020
Available Online: 10 November 2020

Figures(4)

A novel photoenzyme-coupled artificial catalytic system is fabricated by immobilizing horseradish peroxidase (HRP) on the Bi₂WO₆ hollow nanospheres via a facile electrostatic self-assembly process. The obtained Bi₂WO₆/HRP sample not only improves the visible light harvest ability but also promotes the high-efficiency separation of charge carriers. More importantly, the photogenerated electrons and produced H₂O₂ on Bi₂WO₆ directly take part in redox cycle reactions of HRP to induce photoenzyme synergic catalytic effect. In consequence, the degradation activity of Bi₂WO₆/HRP is significantly improved relative to Bi₂WO₆ and HRP for removing bisphenol A (BPA) under the visible light irradiation. This work launches a feasible design strategy for exploiting photoenzyme-coupled artificial catalytic system with special structure to degrade organic pollutants in water efficiently.
- Photoenzyme-coupled,
- Synergistic catalytic effect,
- BPA degradation,
- Reaction mechanism
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Fabrication of HRP/Bi2WO6 photoenzyme-coupled artificial catalytic system for efficiently degrading bisphenol A

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通讯作者: 陈斌, bchen63@163.com

Fabrication of HRP/Bi₂WO₆ photoenzyme-coupled artificial catalytic system for efficiently degrading bisphenol A