Citation: Si Qi-Shi, Guo Wan-Qian, Wang Hua-Zhe, Liu Bang-Hai, Ren Nan-Qi. Carbon quantum dots-based semiconductor preparation methods, applications and mechanisms in environmental contamination[J]. Chinese Chemical Letters, ;2020, 31(10): 2556-2566. doi: 10.1016/j.cclet.2020.08.036 shu

Carbon quantum dots-based semiconductor preparation methods, applications and mechanisms in environmental contamination

State Key Laboratory of Urban Water Resource and Environment, Harbin Institute of Technology, Harbin 150090, China

guowanqian@hit.edu.cn

Received Date: 25 July 2020
Revised Date: 17 August 2020
Accepted Date: 21 August 2020
Available Online: 23 August 2020

Figures(6)

Photocatalyst is the most widespread method in advanced oxidation technologies, but due to the photo-induced electron combine easily with hole and the wavelength of adsorption is limited which will affect some practical applications. Carbon quantum dots (CQDs) is non-toxic and harmless green materials, it has the ability to improve the photocatalytic effect which is attributed to its good electrical and optical properties. Their up-conversion effect, photosensitization and electrical conductivity are assistants which help promote the photocatalytic effect in environmental applications. The key mechanisms of CQDs to improve photocatalysis can be roughly divided into three categories: 1) Up-conversion effect converts the incident light into the emitted light with high energy to solve the problem which is the light absorption range; 2) CQDs act as a photosensitizer instead of valence band to provide electrons to the conduction band of semiconductor; 3) CQDs can be used as the internal or external electronic conductor in materials to alleviate the trend of electron and hole separation. However, CQDs and CQDs-based photocatalysts have different views to solve environmental problems, so it is necessary to integrate different views. Therefore, this review is mainly aimed at the recent researches about the preparation processes of CQD, CQDs-based photocatalysts, and their ability to remove environmental pollutants, with a special emphasis on the mechanism for depredating pollutants. Furthermore, this paper analyzes and discusses the prospects and challenges of CQDs in the environmental field.
- CQDs,
- CQDs modified semiconductor,
- Photodegradation,
- Environmental treatment,
- Photoactive mechanism
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沈阳化工大学材料科学与工程学院沈阳 110142