Citation: Feng Tao, Bavumiragira Jean Pierre, Wambui Mumbi Anne, Kabtamu Daniel Manaye, László Krisztina, Wang Ying, Li Fengting. Hierarchical porous induced competent removal of low concentration azo dye molecules by generating a leachy crystalline structure H-MIL-53(Fe)[J]. Chinese Chemical Letters, ;2020, 31(10): 2717-2720. doi: 10.1016/j.cclet.2020.04.044 shu

Hierarchical porous induced competent removal of low concentration azo dye molecules by generating a leachy crystalline structure H-MIL-53(Fe)

a.
State Key Laboratory of Pollution Control and Resources Reuse, College of Environmental Science and Engineering, Tongji University, Shanghai 200092, China
b.
Shanghai Institute of Pollution Control and Ecological Security, Shanghai 200092, China
c.
Department of Physical Chemistry and Materials Science, Budapest University of Technology and Economics, H-1521 Budapest, Hungary

yingwang@tongji.edu.cn

fengting@tongji.edu.cn

Received Date: 14 February 2020
Revised Date: 2 April 2020
Accepted Date: 24 April 2020
Available Online: 5 May 2020

Figures(4)

The development in technology of synthetic azo dyes, has led to excessive water resources pollution. Even at lower concentration they can impart the quality of water and human life. Herein, we have developed a novel synthesis strategy via introducing salicylic acid (SA) for the synthesis of a leachy crystalline material H-MIL-53(Fe) with hierarchical pores (HP) and exposed coordination unsaturated sites (CUS), which had higher surface area and larger pore volume than the as synthesized MIL-53(Fe). Due to these characteristics, H-MIL-53(Fe) was competent removal of orange G (OG, one of the frequently used azo dyes) with equilibrium in 300 min and the maximum adsorption capacity of 163.9 mg/g. The adsorption mechanism of OG onto H-MIL-53(Fe) was mostly based on electrostatic attraction between CUS of H-MIL-53(Fe) along with HP as active species to OG diffusion and bind. By comparing H-MIL-53(Fe) with other adsorbents for OG adsorption, it is undoubtedly that H-MIL-53(Fe) can be used as a promising adsorbent for OG removal from aqueous solutions.
- H-MIL-53(Fe),
- Salicylic acid,
- Leachy crystalline,
- Adsorption,
- Orange G removal
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1.
沈阳化工大学材料科学与工程学院沈阳 110142