Citation: Zhong Weiming, Zhang Yuyu, Zhao Ling, Li Wanbin. Highly stable and antifouling graphene oxide membranes prepared by bio-inspired modification for water purification[J]. Chinese Chemical Letters, ;2020, 31(10): 2651-2656. doi: 10.1016/j.cclet.2020.03.033 shu

Highly stable and antifouling graphene oxide membranes prepared by bio-inspired modification for water purification

Guangdong Key Laboratory of Environmental Pollution and Health, School of Environment, Jinan University, Guangzhou 511443, China

gandeylin@126.com

Received Date: 3 February 2020
Revised Date: 20 February 2020
Accepted Date: 11 March 2020
Available Online: 12 March 2020

Figures(4)

Graphene oxide (GO) membranes show great potential in molecular separation for water treatment. However, the inferior stability of GO membranes is a major bottleneck for practical applications. In this study, bio-inspired polydopamine (PDA) deposition is reported for enhancing the stability of GO membranes. Through simple and mild immersion, PDA is self-polymerized on GO membranes. The blocking of PDA chains to membrane defects improves the rejections for various molecules. Because the inherently strong adhesion and crosslinking of PDA greatly strengthen the interactions of substrates to GO layers and the binding force of GO nanosheets, the prepared PDA-GO membranes exhibit impressive long-term stability in cross-flow filtration, and maintain good nanofiltration performance at various feed pressures, tangential velocities, and even after external scratching. Moreover, because the deposited PDA layers obstruct the direct contact between GO and contaminants, the antifouling property of the PDA-GO membranes increases substantially, with recovery ratio about 98%.
- Graphene oxide,
- Nanofiltration,
- Polydopamine,
- Stability,
- Antifouling
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沈阳化工大学材料科学与工程学院沈阳 110142