Citation: Li Hao, Gong Jiangfeng, Li Jing-Chang, Zhang Xincheng, Tang Chunmei, Yao Hongbing, Ding Qingping. Synthesis of nickel selenide thin films for high performance all-solid-state asymmetric supercapacitors[J]. Chinese Chemical Letters, ;2020, 31(9): 2275-2279. doi: 10.1016/j.cclet.2020.03.010 shu

Synthesis of nickel selenide thin films for high performance all-solid-state asymmetric supercapacitors

a.
College of Science, Hohai University, Nanjing 210098, China
b.
Ames Laboratory, US DOE, Ames, IA 50011, United States

jfgong@hhu.edu.cn

tcmnj@163.com

Received Date: 28 December 2019
Revised Date: 20 January 2020
Accepted Date: 3 March 2020
Available Online: 4 March 2020

Figures(4)

As a significant semiconductor, nickel selenide shows enormous potential and extensive application prospects in the field of sensor, photocatalysis and supercapacitor. In this paper, nickel selenide (Ni₃Se₂, NiSe) thin films were successfully fabricated on stainless-steel sheet using a facile, effective electrodeposition technique. The morphologies, microstructures and chemical compositions of the thin films are characterized systematically. Electrochemical tests exhibit that the Ni₃Se₂ and NiSe possess high specific capacitance of 581.1 F/g and 1644.7 F/g, respectively. A flexible, all-solid-state asymmetric supercapacitor is assembled by utilizing NiSe film as positive electrode and activated carbon as negative electrode. The solid device delivers a high areal capacitance of 27.0 mF/cm² at the current density of 0.7 mA/cm². The maximum volumetric energy density and power density of the NiSe//AC asymmetric SCs can achieve 0.26 mWh/cm³ and 33.35 mW/cm³, respectively. The device shows robust cycling stability with 84.6% capacitance retention after 10, 000 cycles, outstanding flexibility and satisfactory mechanical stability. Moreover, two devices in series can light up a red light-emitting diode, which displayed great potential applications for energy storage.
- Nickel selenide,
- Electrochemical properties,
- Asymmetric,
- All-solid-state,
- Supercapacitors
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