Citation: Liu Jun, Zhang Cancan, Zhang Shaoxuan, Yu Huajiang, Xie Wei. A versatile β-cyclodextrin functionalized silver nanoparticle monolayer for capture of methyl orange from complex wastewater[J]. Chinese Chemical Letters, ;2020, 31(2): 539-542. doi: 10.1016/j.cclet.2019.07.037 shu

A versatile β-cyclodextrin functionalized silver nanoparticle monolayer for capture of methyl orange from complex wastewater

Liu Jun ^a,1 ,
Zhang Cancan ^a,1 ,
Zhang Shaoxuan ^a,1 ,
Yu Huajiang ^b ,
Xie Wei ^a,*,

a.
Key Lab of Advanced Energy Materials Chemistry (Ministry of Education), Renewable Energy Conversion and Storage Center, College of Chemistry, Nankai University, Tianjin 300071, China
b.
College of Chemistry, State Key Laboratory of Elemento-Organic Chemistry, Nankai University, Tianjin 300071, China

wei.xie@nankai.edu.cn

Received Date: 16 May 2019
Revised Date: 13 July 2019
Accepted Date: 16 July 2019
Available Online: 17 July 2019

Figures(4)

The toxic organic dye contaminants in wastewater are extremely harmful to the ecosystem. Surface enhanced Raman scattering (SERS) is a technique with high sensitivity and chemical specificity which fulfills the requirements for monitoring dye contaminants in wastewater. However, as one of the common dye contaminants, methyl orange (MO) has very weak affinity to metallic surfaces and is difficult to be detected by SERS at low concentrations. Therefore, a new type of SERS substrate with Ag nanoparticle monolayer functionalized by mono-6-deoxy-6-thio-β-cyclodextrin (β-CD-SH) was prepared to efficiently capture and detect MO in wastewater with a limit of detection of 5×10^-7 mol/L. The hydrophobic cavity of β-CD is responsible for the efficient trap and enrichment of MO on the Ag NPs surface, achieving a strong SERS signal of MO at low concentrations and at different pH values. This study provides new insight into designing a well-performed adsorbent for the capture and detection of organic contaminants.
- Dye contaminants,
- Methyl orange,
- SERS,
- Cyclodextrin,
- Wastewater
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