Citation: Teng Zhiwei, Wang Bingtao, Hu Yingying, Xu Danqian. Light-responsive nanocomposites combining graphene oxide with POSS based on host-guest chemistry[J]. Chinese Chemical Letters, ;2019, 30(3): 717-720. doi: 10.1016/j.cclet.2018.08.017 shu

Light-responsive nanocomposites combining graphene oxide with POSS based on host-guest chemistry

Teng Zhiwei ^a,b ,
Wang Bingtao ^b,*, ,
Hu Yingying ^a,b ,
Xu Danqian ^a

a.
State Key Laboratory Breeding Base of Green Chemistry-Synthesis Technology, Zhejiang University of Technology, Hangzhou 310014, China
b.
Institute of Packaging Engineering, Ningbo Institute of Technology, Zhejiang University, Ningbo 315100, China

wbtlion@126.com

Received Date: 27 July 2018
Revised Date: 22 August 2018
Accepted Date: 30 August 2018
Available Online: 31 March 2018

Figures(4)

Based on the reversible host-guest inclusion/exclusion of cyclodextrin-functionalized graphene oxide (GO-CD) and azobenzene-terminated polyhedral oligomeric silsesquioxane (Azo-POSS), a novel kind of light-responsive nanocomposites GO-POSS was developed under mild condition. ¹H NMR, FT-IR, TG, TEM and UV-vis spectroscopy were conducted to characterize the chemical composition and photoresponsive performance of obtained GO-POSS nanocomposites. The results demonstrated that nanocagestructured POSS and nanosheet GO components in GO-POSS exhibited pronounced supramolecular assembly/disassembly behavior upon UV/vis irradiation. Moreover, GO-POSS nanocomposites showed good water dispersity and had remarkable impact on oxygen permeability of conventional PVA-coated films under varied light irradiation conditions, which would be valuable for developing smart gas barrier materials in packaging.
- Graphene oxide,
- POSS,
- Light-responsiveness,
- Host-guest inclusion,
- Oxygen permeability
1. [1]
  S. Guragain, B.P. Bastakoti, V. Malgras, et al., Chem.-Eur. J. 21 (2015) 13164-13174. doi: 10.1002/chem.v21.38
2. [2]
  L. Yang, W. Xiaowen, F. Bin, et al., Adv. Funct. Mater. 25 (2015) 5047-5056. doi: 10.1002/adfm.v25.31
3. [3]
  E.G. Kelley, J.N.L. Albert, M.O. Sullivan, et al., Chem. Soc. Rev. 42 (2013) 7057-7071. doi: 10.1039/c3cs35512h
4. [4]
  P. Kaner, X. Hu, S.W. Thomas, et al., ACS Appl. Mater. Interfaces 9 (2017) 13619-13631. doi: 10.1021/acsami.7b01585
5. [5]
  W. Lee, D. Kim, J. Lim, et al., Sens. Actuators B 266 (2018) 724-729. doi: 10.1016/j.snb.2018.03.166
6. [6]
  M.L. Wei, Y.F. Gao, X. Li, et al., Polym. Chem. 8 (2017) 127-143. doi: 10.1039/C6PY01585A
7. [7]
  O. Bertrand, J.F. Gohy, Polym. Chem. 8 (2017) 52-73. doi: 10.1039/C6PY01082B
8. [8]
  J.F. Gohy, Y. Zhao, Chem. Soc. Rev. 42 (2013) 7117-7129. doi: 10.1039/c3cs35469e
9. [9]
  L.N. Fu, B. Leng, Y.S. Li, et al., Chin. Chem. Lett. 27 (2016) 1319-1329. doi: 10.1016/j.cclet.2016.06.045
10. [10]
  K.Y. Chun, Y.J. Son, S. Jo, C.S. Han, Small 14 (2018) 1703618.
11. [11]
  K. Ke, Z.K. Du, X.Y. Chang, et al., Colloid Polym. Sci. 295 (2017) 1851-1861. doi: 10.1007/s00396-017-4156-z
12. [12]
  X.J. Liao, G.S. Chen, Chin. Chem. Lett. 27 (2016) 583-587. doi: 10.1016/j.cclet.2016.02.022
13. [13]
  X.J. Zhang, X. Ma, K. Wang, et al., Macromol. Rapid Commun. 39 (2018) 1800142.
14. [14]
  B.W. Liu, H. Zhou, S.T. Zhou, et al., Eur. Polym. J. 65 (2015) 63-81. doi: 10.1016/j.eurpolymj.2015.01.017
15. [15]
  P. Shi, E. Ju, Z. Yan, et al., Nat. Commun. 7 (2016) 13088.
16. [16]
  C.N.R. Rao, A.K. Sood, K.S. Subrahmanyam, et al., Angew. Chem. Int. Ed. 48 (2009) 7752-7777. doi: 10.1002/anie.v48:42
17. [17]
  A.K. Geim, Science 324 (2009) 1530-1534. doi: 10.1126/science.1158877
18. [18]
  K. Tanaka, Y. Chujo, J. Mater. Chem. 22 (2012) 1733-1746. doi: 10.1039/C1JM14231C
19. [19]
  G. Potsi, A. Rossos, A. Kouloumpis, et al., Curr. Org. Chem. 20 (2016) 662-673. doi: 10.2174/1385272819666151006010352
20. [20]
  Y.N. Lu, S.L. Zhang, Z. Geng, et al., New J. Chem. 41 (2017) 3089-3096. doi: 10.1039/C6NJ03802F
21. [21]
  Y.J. Guo, S.J. Guo, J.T. Ren, et al., ACS Nano 4 (2010) 4001-4010. doi: 10.1021/nn100939n
22. [22]
  O.C. Compton, S. Kim, C. Pierre, et al., Adv. Mater. 22 (2010) 4759-4763. doi: 10.1002/adma.v22:42
23. [23]
  Y.B. Cui, S.I. Kundalwal, S. Kumar, Carbon 98 (2016) 313-333. doi: 10.1016/j.carbon.2015.11.018
24. [24]
  F. Mannle, T.R. Tofteberg, M. Skaugen, et al., J. Nanopart. Res. 13 (2011) 4691-4701. doi: 10.1007/s11051-011-0435-7
25. [25]
  P. Iyer, G. Iyer, M. Coleman, J. Membr. Sci. 358 (2010) 26-32.
1. [1]
  Yuanyi Zhou , Ke Ma , Jinfeng Liu , Zirun Zheng , Bo Hu , Yu Meng , Zhizhong Li , Mingshan Zhu . Is reactive oxygen species the only way for cancer inhibition over single atom nanomedicine? Autophagy regulation also works. Chinese Chemical Letters, 2024, 35(6): 109056-. doi: 10.1016/j.cclet.2023.109056
2. [2]
  Ying Chen , Li Li , Junyao Zhang , Tongrui Sun , Xuan Zhang , Shiqi Zhang , Jia Huang , Yidong Zou . Tailored ionically conductive graphene oxide-encased metal ions for ultrasensitive cadaverine sensor. Chinese Chemical Letters, 2024, 35(8): 109102-. doi: 10.1016/j.cclet.2023.109102
3. [3]
  Tian TIAN , Meng ZHOU , Jiale WEI , Yize LIU , Yifan MO , Yuhan YE , Wenzhi JIA , Bin HE . Ru-doped Co₃O₄/reduced graphene oxide: Preparation and electrocatalytic oxygen evolution property. Chinese Journal of Inorganic Chemistry, 2025, 41(2): 385-394. doi: 10.11862/CJIC.20240298
4. [4]
  Jianmei Guo , Yupeng Zhao , Lei Ma , Yongtao Wang . Ultra-long room temperature phosphorescence, intrinsic mechanisms and application based on host-guest doping systems. Chinese Journal of Structural Chemistry, 2024, 43(9): 100335-100335. doi: 10.1016/j.cjsc.2023.100335
5. [5]
  Jie Yang , Xin-Yue Lou , Dihua Dai , Jingwei Shi , Ying-Wei Yang . Desymmetrized pillar[8]arenes: High-yield synthesis, functionalization, and host-guest chemistry. Chinese Chemical Letters, 2025, 36(1): 109818-. doi: 10.1016/j.cclet.2024.109818
6. [6]
  Jia-Li Xie , Tian-Jin Xie , Yu-Jie Luo , Kai Mao , Cheng-Zhi Huang , Yuan-Fang Li , Shu-Jun Zhen . Octopus-like DNA nanostructure coupled with graphene oxide enhanced fluorescence anisotropy for hepatitis B virus DNA detection. Chinese Chemical Letters, 2024, 35(6): 109137-. doi: 10.1016/j.cclet.2023.109137
7. [7]
  Yihong Li , Zhong Qiu , Lei Huang , Shenghui Shen , Ping Liu , Haomiao Zhang , Feng Cao , Xinping He , Jun Zhang , Yang Xia , Xinqi Liang , Chen Wang , Wangjun Wan , Yongqi Zhang , Minghua Chen , Wenkui Zhang , Hui Huang , Yongping Gan , Xinhui Xia . Plasma enhanced reduction method for synthesis of reduced graphene oxide fiber/Si anode with improved performance. Chinese Chemical Letters, 2024, 35(11): 109510-. doi: 10.1016/j.cclet.2024.109510
8. [8]
  Jincheng Zhang , Mengjie Sun , Jiali Ren , Rui Zhang , Min Ma , Qingzhong Xue , Jian Tian . Oxygen vacancies-rich molybdenum tungsten oxide nanowires as a highly active nitrogen fixation electrocatalyst. Chinese Chemical Letters, 2025, 36(1): 110491-. doi: 10.1016/j.cclet.2024.110491
9. [9]
  Xin Wang , Changzhao Chen , Qishen Wang , Kai Dai . Graphene quantum dot modified Bi2MoO6 nanoflower for efficient degradation of BPA under visible light. Chinese Journal of Structural Chemistry, 2024, 43(12): 100473-100473. doi: 10.1016/j.cjsc.2024.100473
10. [10]
  Hao Cai , Xiaoyan Wu , Lei Jiang , Feng Yu , Yuxiang Yang , Yan Li , Xian Zhang , Jian Liu , Zijian Li , Hong Bi . Lysosome-targeted carbon dots with a light-controlled nitric oxide releasing property for enhanced photodynamic therapy. Chinese Chemical Letters, 2024, 35(4): 108946-. doi: 10.1016/j.cclet.2023.108946
11. [11]
  Bingbing Shi , Yuchun Wang , Yi Zhou , Xing-Xing Zhao , Yizhou Li , Nuoqian Yan , Wen-Juan Qu , Qi Lin , Tai-Bao Wei . A supramolecular oligo[2]rotaxane constructed by orthogonal platinum(Ⅱ) metallacycle and pillar[5]arene-based host–guest interactions. Chinese Chemical Letters, 2024, 35(10): 109540-. doi: 10.1016/j.cclet.2024.109540
12. [12]
  Mengxiang Zhu , Tao Ding , Yunzhang Li , Yuanjie Peng , Ruiping Liu , Quan Zou , Leilei Yang , Shenglei Sun , Pin Zhou , Guosheng Shi , Dongting Yue . Graphene controlled solid-state growth of oxygen vacancies riched V₂O₅ catalyst to highly activate Fenton-like reaction. Chinese Chemical Letters, 2024, 35(12): 109833-. doi: 10.1016/j.cclet.2024.109833
13. [13]
  Yan Wang , Huixin Chen , Fuda Yu , Shanyue Wei , Jinhui Song , Qianfeng He , Yiming Xie , Miaoliang Huang , Canzhong Lu . Oxygen self-doping pyrolyzed polyacrylic acid as sulfur host with physical/chemical adsorption dual function for lithium-sulfur batteries. Chinese Chemical Letters, 2024, 35(7): 109001-. doi: 10.1016/j.cclet.2023.109001
14. [14]
  Tian Cao , Xuyin Ding , Qiwen Peng , Min Zhang , Guoyue Shi . Intelligent laser-induced graphene sensor for multiplex probing catechol isomers. Chinese Chemical Letters, 2024, 35(7): 109238-. doi: 10.1016/j.cclet.2023.109238
15. [15]
  Rui Liu , Jinbo Pang , Weijia Zhou . Monolayer water shepherding supertight MXene/graphene composite films. Chinese Journal of Structural Chemistry, 2024, 43(10): 100329-100329. doi: 10.1016/j.cjsc.2024.100329
16. [16]
  Ling Tang , Yan Wan , Yangming Lin . Lowering the kinetic barrier via enhancing electrophilicity of surface oxygen to boost acidic oxygen evolution reaction. Chinese Journal of Structural Chemistry, 2024, 43(11): 100345-100345. doi: 10.1016/j.cjsc.2024.100345
17. [17]
  Shenghui Tu , Anru Liu , Hongxiang Zhang , Lu Sun , Minghui Luo , Shan Huang , Ting Huang , Honggen Peng . Oxygen vacancy regulating transition mode of MIL-125 to facilitate singlet oxygen generation for photocatalytic degradation of antibiotics. Chinese Chemical Letters, 2024, 35(12): 109761-. doi: 10.1016/j.cclet.2024.109761
18. [18]
  Hanqing Zhang , Xiaoxia Wang , Chen Chen , Xianfeng Yang , Chungli Dong , Yucheng Huang , Xiaoliang Zhao , Dongjiang Yang . Selective CO2-to-formic acid electrochemical conversion by modulating electronic environment of copper phthalocyanine with defective graphene. Chinese Journal of Structural Chemistry, 2023, 42(10): 100089-100089. doi: 10.1016/j.cjsc.2023.100089
19. [19]
  Qiang Cao , Xue-Feng Cheng , Jia Wang , Chang Zhou , Liu-Jun Yang , Guan Wang , Dong-Yun Chen , Jing-Hui He , Jian-Mei Lu . Graphene from microwave-initiated upcycling of waste polyethylene for electrocatalytic reduction of chloramphenicol. Chinese Chemical Letters, 2024, 35(4): 108759-. doi: 10.1016/j.cclet.2023.108759
20. [20]
  Cheng Guo , Xiaoxiao Zhang , Xiujuan Hong , Yiqiu Hu , Lingna Mao , Kezhi Jiang . Graphene as adsorbent for highly efficient extraction of modified nucleosides in urine prior to liquid chromatography-tandem mass spectrometry analysis. Chinese Chemical Letters, 2024, 35(4): 108867-. doi: 10.1016/j.cclet.2023.108867

Get Citation

PDF

XML

Metrics

PDF Downloads(3)
Abstract views(639)
HTML views(36)

通讯作者: 陈斌, bchen63@163.com

1.
沈阳化工大学材料科学与工程学院沈阳 110142