Citation: Han Chengjie, Tian Zhen, Dou Huanglin, Wang Xiaomin, Yang Xiaowei. Vertical crosslinking MoS₂/three-dimensional graphene composite towards high performance supercapacitor[J]. Chinese Chemical Letters, ;2018, 29(4): 606-611. doi: 10.1016/j.cclet.2018.01.017 shu

Vertical crosslinking MoS₂/three-dimensional graphene composite towards high performance supercapacitor

a.
College of Materials Science and Engineering, Taiyuan University of Technology, Taiyuan 030024, China
b.
Research Institute of Tsinghua University in Shenzhen, Shenzhen 518057, China

Corresponding author: Wang Xiaomin, wangxiaomin@tyut.edu.cn Yang Xiaowei, yang-xw@163.com
Received Date: 9 November 2017
Revised Date: 8 January 2018
Accepted Date: 9 January 2018
Available Online: 10 April 2018

Figures(4)

Molybdenum disulfide (MoS₂) has been stimulated in extensive researches due to its layered structure and the potential as an electrochemical energy material. However, the effects on electrochemical performance of concentration of MoS₂ are rarely mentioned. In this paper, the effects of different concentrated layered MoS₂ on the morphology and electrochemical properties of the composite of MoS₂ and three-dimensional graphene (MoS₂/3DG) were discussed. The results show that layered MoS₂ was successfully compounded to 3DG and formed a vertical crosslinking structure. It can be observed that MoS₂ nanosheets are vertically loaded on the inner and outer surface of graphene when the concentration of MoS₂ is 0.20 mg/L. The specific capacitance of composite (MoS₂ (0.20 mg/L)/3DG) reaches 2182.33 mF/cm² at the current density of 1 mA/cm², and the specific capacitance remains 116.83% after 5000 cycles. When the current density increased 100 times (from 1 mA/cm² to 100 mA/cm²), the specific capacitance retains 78.9%. Meanwhile, the hybrid energy storage devises can deliver an energy density of 130.34 Wh/m². The superior electrochemical properties are attributed to the synergistic effect of MoS₂ and 3DG. Therefore, the material has a potential application on supercapacitor electrode material.
- MoS₂,
- Three-dimensional graphene,
- Supercapacitor,
- Vertical crosslinking,
- Energy storage
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通讯作者: 陈斌, bchen63@163.com

1.
沈阳化工大学材料科学与工程学院沈阳 110142

Vertical crosslinking MoS2/three-dimensional graphene composite towards high performance supercapacitor

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通讯作者: 陈斌, bchen63@163.com

Vertical crosslinking MoS₂/three-dimensional graphene composite towards high performance supercapacitor