Citation: Zhu Yingke, Jiang Pingkai, Zhang Zhicheng, Huang Xingyi. Dielectric phenomena and electrical energy storage of poly(vinylidene fluoride) based high-k polymers[J]. Chinese Chemical Letters, ;2017, 28(11): 2027-2035. doi: 10.1016/j.cclet.2017.08.053 shu

Dielectric phenomena and electrical energy storage of poly(vinylidene fluoride) based high-k polymers

a.
Department of Polymer Science and Engineering, Shanghai Key Laboratory of Electrical Insulation and Thermal Aging, Shanghai Jiao Tong University, Shanghai 200240, China
b.
Department of Applied Chemistry, School of Science, Xi'an Jiaotong University, Xi'an 710049, China

Author Bio:

Zhicheng Zhang, Professor of Xi’an Jiaotong University majored in polymer physics and chemistry, earned his BS and MS degree in polymer materials and engineering in 1999 and 2002 from Xi’an Jiaotong University, and his Ph. D. degree in polymer physics and chemistry in 2005 from Institute of Chemistry, Chinese Academy of Sciences. From 2005 to 2008, he worked as a postdoc in Department of Materials Science and Engineering, Pennsylvania State University, USA. Since 2008, he started to work in Xi’an Jiaotong University as full professor. He is leading a groupfocus onthe synthesis andmodification of fluoropolymers, fabrication of novel electroactive materials for energy generation, transformation and storage. He has published over 80 SCI papers with a citation over 1200 and his personal Hindex is 21. Prof. Zhang is currently regular referee for over 50 polymer and materials journals including Macromolecules, Macromolecular Rapid Communications, Polymer Chemistry, ACS Applied Materials and Interfaces, Journal of Materials Chemistry and Applied Physics Letters. He is member of American Chemical Society and Chinese Chemical Society. In 2010, he was supported by Program for New Century Excellent Talents in University. So far, he has chaired over 20 scientific research programs including two from NSFC
Xingyi Huang, received his Ph.D. degree in 2008 from the Research Center of Dielectric and Electrical Insulation at Shanghai Jiao Tong University. After graduation, he became a staff member in Shanghai Key Laboratory of Electrical Insulation and Thermal Ageing at Shanghai Jiao Tong University, and worked with Prof. Toshikatsu Tanaka at Waseda University as a visiting researcher from 2011 to 2012. Since 2013, he has been an associate professor in Shanghai Key Laboratory of Electrical Insulation and Thermal Ageing and Department of Polymer Science and Engineering at Shanghai Jiao Tong University. Huang was the Winner of NSFC Foundation for Excellent Young Scholars and Winner of Shanghai Pujiang Talent Program. He is an editorial board member of Advanced Composites and Hybrid Materials and IET Nanodielectrics. He was also a Guest Editor of IEEE Transactions on Dielectrics and Electrical Insulation and is an Associate Editor of High Voltage
Corresponding author: Zhang Zhicheng, zhichengzhang@mail.xjtu.edu.cn Huang Xingyi, xyhuang@sjtu.edu.cn
Received Date: 4 May 2017
Revised Date: 23 August 2017
Accepted Date: 30 August 2017
Available Online: 1 November 2017

Figures(18)

Polymeric dielectrics have wide range of applications in the field of electrical energy storage because of their light weight and easy processing. However, the state-of-the-art polymer dielectrics, such as biaxially orientated polypropylene, could not meet the demand of minimization of electronic devices because of its low energy density. Recently, poly(vinylidene fluoride) (PVDF) based ferroelectric polymers have attracted considerable interests for energy storage applications because of their high permittivity and high breakdown strength. Unfortunately, the high dielectric loss and/or high remnant polarization of PVDF-based polymers seriously limits their practical applications for electrical energy storage. Since the discovery of relaxor ferroelectric behavior was firstly reported in irradiated poly(vinylidene fluoridetrifluoroethylene) (P(VDF-TrFE)) copolymer, many strategies have been developed to enhanced the electrical energy storage capability, including copolymerization, grafting, blending and fabricating of multilayer. How these methods affect the polymorphs, crystallinity, crystal size of PVDF-based polymers and the connection between these microstructures and their corresponding energy storage properties are discussed in detail.
- PVDF,
- Ferroelectric polymer,
- Copolymerization,
- Grafting,
- Energy storage,
- Dielectric constant,
- Dielectric loss,
- Breakdown strength
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