FeOOH调节Bi12O17Cl2@FeOOH异质结中Bi12O17Cl2的表面势阱深度以增强压电电荷转移和压电自芬顿催化

引用本文: 邱江源, 于涛, 陈均鑫, 李文轩, 张晓萱, 李金生, 郭瑞, 黄在银, 刘宣文. FeOOH调节Bi₁₂O₁₇Cl₂@FeOOH异质结中Bi₁₂O₁₇Cl₂的表面势阱深度以增强压电电荷转移和压电自芬顿催化[J]. 物理化学学报, 2026, 42(1): 100157. doi: 10.1016/j.actphy.2025.100157 shu

Citation: Jiangyuan Qiu, TaoYu, Junxin Chen, Wenxuan Li, Xiaoxuan Zhang, jinsheng Li, Rui Guo, Zaiyin Huang, Xuanwen Liu. Modulate surface potential well depth of Bi₁₂O₁₇Cl₂ by FeOOH in Bi₁₂O₁₇Cl₂@FeOOH heterojunction to boost piezoelectric charge transfer and piezo-self-Fenton catalysis[J]. Acta Physico-Chimica Sinica, 2026, 42(1): 100157. doi: 10.1016/j.actphy.2025.100157 shu

FeOOH调节Bi₁₂O₁₇Cl₂@FeOOH异质结中Bi₁₂O₁₇Cl₂的表面势阱深度以增强压电电荷转移和压电自芬顿催化

邱江源 ^1,2,3, ,
于涛 ^1,2, ,
陈均鑫 ^3, ,
李文轩 ^3, ,
张晓萱 ^1,2, ,
李金生 ^1,2, ,
郭瑞 ^{1,2,
,} ,
黄在银 ^{3,
,} ,
刘宣文 ^{1,2,
,}

1.
东北大学材料科学与工程学院, 辽宁沈阳 110819;
2.
东北大学秦皇岛分校资源与材料学院, 河北秦皇岛 066004;
3.
广西民族大学化学化工学院, 广西南宁 530006

通讯作者: 郭瑞，Emails:guorui@neuq.edu.cn; 黄在银，Emails:huangzaiyin@163.com; 刘宣文，Emails:lxw@neuq.edu.cn

基金项目:
国家自然科学基金(21873048, 22263001)和秦皇岛市重点研发计划(202302B013)资助项目

摘要: 尽管异质结压电催化剂的设计被证明可以显著提升其催化活性，但异质结界面在压电过程中对表面势阱的调控机制及其对载流子迁移的影响仍缺乏系统研究。本研究通过自组装策略，在Bi₁₂O₁₇Cl₂@FeOOH体系中构建了非晶FeOOH与Bi₁₂O₁₇Cl₂之间的增强界面相互作用异质界面结。这种强界面相互作用显著增强了界面极性，可大幅抑制Bi₁₂O₁₇Cl₂表面电荷的应力响应能力(最大降幅达原始值的63%–98%)，这显著降低了压电过程中表面势阱的深度，从而有效削弱了压电电荷的束缚，同时促进了电荷转移。同时，界面形成的Bi–O–Fe化学键构建了电荷传输通道。这些协同机制使得压电自芬顿反应中H₂O₂产率达到3.04 mmol g⁻¹ h⁻¹，总有机碳去除率提高了3倍(从18.6%增至55.8%)。

关键词:

English

Modulate surface potential well depth of Bi₁₂O₁₇Cl₂ by FeOOH in Bi₁₂O₁₇Cl₂@FeOOH heterojunction to boost piezoelectric charge transfer and piezo-self-Fenton catalysis

1.
School of Materials Science and Engineering, Northeastern University, Shenyang 110819, Liaoning Province, China;
2.
School of Resources and Materials, Northeastern University at Qinhuangdao, Qinhuangdao 066004, Hebei Province, China;
3.
School of Chemistry and Chemical Engineering, Guangxi Minzu University, Nanning 530006, Guangxi Zhuang Autonomous Region, China

Corresponding author: Rui Guo, ; Zaiyin Huang, ; Xuanwen Liu,

Received Date: 24 May 2025
Revised Date: 10 August 2025
Available Online: 13 August 2025

Abstract: Although the design of heterojunction piezoelectric catalysts has significantly enhanced catalytic activity, the regulatory mechanisms of heterojunction interfaces on surface potential wells during piezoelectric processes and their impact on carrier migration still lack systematic investigation. This work constructs an enhance interface interaction heterointerface between amorphous FeOOH and Bi₁₂O₁₇Cl₂ (BOC) in Bi₁₂O₁₇Cl₂@FeOOH through a self-assembly strategy. ‌This strong interfacial interaction significantly enhances interface polarity can substantially suppress the stress-responsive capability of surface charges on BOC (maximum reduction reached as high as 63%–98% of original value). This significantly reduces the depth of surface potential wells during piezoelectric processes, thereby effectively weakening piezoelectric charge confinement while promoting charge transfer. Concurrently, Bi–O–Fe chemical bonds formed at the interface and establish charge transport channels. These synergistic mechanisms elevate the H₂O₂ production rate to 3.04 mmol g⁻¹ h⁻¹ for participate in the piezoelectric self-Fenton reaction and the removal rate of total organic carbon increased 3 fold (18.6% vs. 55.8%).

Key words:

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沈阳化工大学材料科学与工程学院沈阳 110142

FeOOH调节Bi₁₂O₁₇Cl₂@FeOOH异质结中Bi₁₂O₁₇Cl₂的表面势阱深度以增强压电电荷转移和压电自芬顿催化

通讯作者: 郭瑞，Emails:guorui@neuq.edu.cn; 黄在银，Emails:huangzaiyin@163.com; 刘宣文，Emails:lxw@neuq.edu.cn

English

Modulate surface potential well depth of Bi₁₂O₁₇Cl₂ by FeOOH in Bi₁₂O₁₇Cl₂@FeOOH heterojunction to boost piezoelectric charge transfer and piezo-self-Fenton catalysis

Corresponding author: Rui Guo, ; Zaiyin Huang, ; Xuanwen Liu,

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