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设计串联S型光催化体系：机理见解、表征技术与应用

KumarRohit ,  SudhaikAnita ,  Pawaz KhanAftab Asalam ,  NeguyenVan Huy ,  SinghArchana ,  SinghPardeep ,  ThakurSourbh ,  RaizadaPankaj

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引用本文: KumarRohit, SudhaikAnita, Pawaz KhanAftab Asalam, NeguyenVan Huy, SinghArchana, SinghPardeep, ThakurSourbh, RaizadaPankaj. 设计串联S型光催化体系：机理见解、表征技术与应用[J]. 物理化学学报, 2025, 41(11): 100150. doi: 10.1016/j.actphy.2025.100150 shu
Citation:  Rohit Kumar, Anita Sudhaik, Aftab Asalam Pawaz Khan, Van Huy Neguyen, Archana Singh, Pardeep Singh, Sourbh Thakur, Pankaj Raizada. Designing tandem S-scheme photo-catalytic systems: Mechanistic insights, characterization techniques, and applications[J]. Acta Physico-Chimica Sinica, 2025, 41(11): 100150. doi: 10.1016/j.actphy.2025.100150 shu

设计串联S型光催化体系：机理见解、表征技术与应用

  • 1.

    School of Advanced Chemical Sciences, Shoolini University, Solan, HP 173229, India

  • 2.

    Center of Excellence for Advanced Materials Research, King Abdulaziz University, Jeddah 21589, Saudi Arabia

  • 3.

    Chettinad Hospital and Research Institute, Chettinad Academy of Research and Education (CARE), Kelambakkam, Kanchipuram District, 603103, Tamil Nadu, India

  • 4.

    Advanced Materials and Processes Research Institute, Hoshangabad Road, Bhopal, 462026, MP, India

  • 5.

    Department of Organic Chemistry, Bioorganic Chemistry and Biotechnology, Silesian University of Technology, B. Krzywoustego 4, 44-100 Gliwice, Poland

    • 通讯作者: SinghPardeep, pardeepchem@gmail.com; RaizadaPankaj, pankajchem1@gmail.com
摘要: 串联S型异质结已成为光催化领域一项极具前景的创新技术，为环境修复提供了有效解决方案。与传统Z型或Ⅱ型光催化剂不同，S型结构选择性保留了高效参与氧化还原反应的高能光生载流子。这种独特机理能增强电荷分离、强化内建电场并提升光吸收能力。然而，单结S型体系存在量子效率低的问题。因此，构建多组分S型体系可有效提升光催化性能。串联S型体系由多个具有交错能带位置的半导体/材料组成，形成阶梯式或定向电荷转移机制。这种阶梯式电位梯度可显著提升电荷分离、光吸收、氧化还原能力、稳定性及整体光催化活性。本文深入阐述了串联S型异质结的作用原理，探讨了通过半导体配对、助催化剂添加和介质嵌入等设计策略实现电荷迁移最大化与复合最小化的方法；系统分析了多种合成路径及其动力学与热力学原理；讨论了包括密度泛函理论(DFT)模拟、原位X射线光电子能谱(XPS)、瞬态吸收光谱(TAS)、光致发光(PL)和电化学阻抗谱(EIS)在内的一系列先进表征手段，这些技术为揭示电子行为与界面动力学提供了重要见解。文章还探讨了该类异质结在二氧化碳还原、产氢和有机污染物降解等主要领域的应用。尽管潜力显著，但仍需解决合成工艺复杂、材料稳定性和规模化生产等挑战。针对现有局限，本文提出了未来研究方向。总体而言，串联S型异质结是构建高效可持续光催化技术的卓越方案。

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