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瞬态吸收光谱在太阳能转化利用中的研究进展

张凤英 ,  梅杨林 ,  蒋毓蔓 ,  郑申申 ,  郑凯波 ,  周莹

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引用本文: 张凤英, 梅杨林, 蒋毓蔓, 郑申申, 郑凯波, 周莹. 瞬态吸收光谱在太阳能转化利用中的研究进展[J]. 物理化学学报, 2025, 41(9): 100118. doi: 10.1016/j.actphy.2025.100118 shu
Citation:  Fengying Zhang, Yanglin Mei, Yuman Jiang, Shenshen Zheng, Kaibo Zheng, Ying Zhou. Research progress of transient absorption spectroscopy in solar energy conversion and utilization[J]. Acta Physico-Chimica Sinica, 2025, 41(9): 100118. doi: 10.1016/j.actphy.2025.100118 shu

瞬态吸收光谱在太阳能转化利用中的研究进展

  • 1.

    西南石油大学, 氢能绿色制储与高效利用川渝共建重点实验室, 四川 成都 610500

  • 2.

    西南石油大学新能源与材料学院, 四川 成都 610500

  • 3.

    Department of Chemical Physics and NanoLund Chemical Center, Lund University, Lund 22100, Sweden

  • 4.

    Department of Chemistry, Technical University of Denmark, Kongens Lyngby DK-2800, Denmark

    • 通讯作者: 周莹, yzhou@swpu.edu.cn
  • 基金项目:

    国家重点研发项目 2020YFA0710000

    国家自然科学基金项目 52325401

    国家自然科学基金项目 22309152

    国家自然科学基金项目 22311530118

    四川省重点研发项目 2024YFHZ0040

    四川省高端外国专家引进计划项目 2025HJRC0018

    成都市国际科技合作项目 2021-GH02-00052-HZ

摘要: 随着超快激光技术的不断发展，时间分辨光谱技术已成为研究太阳能转化与利用领域中超快时间尺度下微观光物理机制的重要工具。瞬态吸收光谱(Transient Absorption Spectroscopy, TAS)作为研究光诱导超快电子转移与载流子动力学过程的重要技术，具有揭示光生载流子产生、分离、传输及复合等关键动力学过程的独特优势。本文围绕光-化学能转换和光-电能转换，概述了TAS技术在光催化和太阳能电池两大主要太阳能转化与利用领域的应用。首先，根据光催化(侧重载流子迁移参与表面反应)与太阳能电池(强调载流子界面分离效率)对载流子的不同需求，分别从电子调控、空穴调控和表界面过程三个方面概括了促进载流子迁移利用的设计策略与研究进展。然后，特别关注了原位光谱在光-电-热等复杂应用条件下对能源转换微观过程及性能的影响机制。最后，总结了对太阳能转化与利用领域基础研究的前瞻性发展方向，为太阳能转化材料、反应、器件的理性设计与性能优化提供理论支持。

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