Citation: Fengying Zhang, Yanglin Mei, Yuman Jiang, Shenshen Zheng, Kaibo Zheng, Ying Zhou. Research progress of transient absorption spectroscopy in solar energy conversion and utilization[J]. Acta Physico-Chimica Sinica, ;2025, 41(9): 100118. doi: 10.1016/j.actphy.2025.100118 shu

Research progress of transient absorption spectroscopy in solar energy conversion and utilization

Fengying Zhang ^{1, 2} ,
Yanglin Mei ¹ ,
Yuman Jiang ¹ ,
Shenshen Zheng ¹ ,
Kaibo Zheng ^{3, 4} ,
Ying Zhou ^{1, 2,,}

1.
Sichuan-Chongqing Joint Key Laboratory of Green Hydrogen Production & Storage and Efficient Utilization, Chengdu 610500, Sichuan Province, China
2.
School of New Energy and Materials, Southwest Petroleum University, Chengdu 610500, Sichuan Province, China
3.
Department of Chemical Physics and NanoLund Chemical Center, Lund University, Lund 22100, Sweden
4.
Department of Chemistry, Technical University of Denmark, Kongens Lyngby DK-2800, Denmark

Corresponding author: Ying Zhou, yzhou@swpu.edu.cn
Received Date: 24 April 2025
Revised Date: 9 June 2025
Accepted Date: 10 June 2025

Fund Project: the National Key R&D Project of China 2020YFA0710000the National Natural Science Foundation of China 52325401the National Natural Science Foundation of China 22309152the National Natural Science Foundation of China 22311530118the Provincial Key Research and Development Project of Sichuan 2024YFHZ0040the High-end Foreign Experts Recruitment Program Sichuan 2025HJRC0018the International Science and Technology Cooperation Project of Chengdu 2021-GH02-00052-HZ

With the development of ultrafast laser technology, time-resolved spectroscopy has become an essential tool to study the microscopic photophysical mechanisms on ultrafast time scales in the field of solar energy conversion and utilization. Transient absorption spectroscopy (TAS), as an essential technology for studying photoinduced ultrafast electron transfer and photo-induced carrier dynamics, has the unique advantage of revealing key dynamic processes, such as the generation, separation, transport, and recombination of photogenerated carriers. Focusing on light-to-chemical and light-to-electrical energy conversion, this review summarizes TAS applications in two primary solar energy conversion systems: photocatalysis and solar cells. Firstly, according to the different requirements of photocatalysis (emphasizing migration for surface reactions) and solar cells (highlighting interfacial carrier separation efficiency), we summarize design strategies and recent advances for enhancing carrier utilization from three perspectives: electron manipulation, hole manipulation and surface interfacial processes. Subsequently, special attention is given to how in situ spectroscopy elucidates the influence mechanisms of microscopic energy conversion processes and device performance under complex application scenarios involving photo-electro-thermal couplings. Finally, the forward-looking development direction of basic research in solar energy conversion and utilization is summarized, which provides theoretical support for rational design and performance optimization of solar energy conversion materials, reactions, and devices.
- Solar energy conversion and utilization,
- Transient absorption spectroscopy,
- Photocatalysis,
- Solar cells,
- In situ spectroscopy
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