Citation: Xintong Zhu, Bin Cao, Chong Yan, Cheng Tang, Aibing Chen, Qiang Zhang. Advances in coating strategies for graphite anodes in lithium-ion batteries[J]. Acta Physico-Chimica Sinica, ;2025, 41(9): 100096. doi: 10.1016/j.actphy.2025.100096 shu

Advances in coating strategies for graphite anodes in lithium-ion batteries

Xintong Zhu ^{1, 2} ,
Bin Cao ^{2, 3} ,
Chong Yan ⁴ ,
Cheng Tang ^{2, 5,,} ,
Aibing Chen ^1,, ,
Qiang Zhang ^{2, 6,,}

1.
College of Chemical and Pharmaceutical Engineering, Hebei University of Science and Technology, Shijiazhuang 050018, China
2.
Beijing Key Laboratory of Complex Solid State Batteries & Tsinghua Center for Green Chemical Engineering Electrification, Department of Chemical Engineering, Tsinghua University, Beijing 100084, China
3.
College of Materials Science and Engineering, Xi'an University of Science and Technology, Xi'an 710054, China
4.
Advanced Research Institute of Multidisciplinary Science, Beijing Institute of Technology, Beijing 100081, China
5.
Ordos Laboratory, Ordos 017000, Inner Mongolia Autonomous Region, China
6.
Institute for Carbon Neutrality, Tsinghua University, Beijing 100084, China

Corresponding author: Cheng Tang, cheng–net0@tsinghua.edu.cn Aibing Chen, chen_ab@163.com Qiang Zhang, zhang–qiang@mails.tsinghua.edu.cn
Received Date: 5 March 2025
Revised Date: 11 April 2025
Accepted Date: 18 April 2025

Fund Project: the National Key Research and Development Program of China 2022YFB2404402Huaneng Group science and technology research project HNKJ23–H71National Natural Science Foundation of China 22478221National Natural Science Foundation of China U23A20573National Natural Science Foundation of China U23A20140the Hebei Natural Science Foundation B2024208091S&T Program of Hebei 22344402D

As a critical component for achieving sustainable energy systems, secondary lithium-ion batteries (LIBs) have become the dominant electrochemical energy storage technology. Graphite has been widely employed as an anode material in rechargeable LIBs, where the formation of a solid electrolyte interphase (SEI) on graphite particles plays a pivotal role in realizing optimal Li⁺ ion storage performance. However, solvent co-intercalation with Li⁺ ions leads to volumetric expansion, unstable SEI formation, irreversible capacity loss, structural layer collapse, and even lithium dendrite formation. To overcome these challenges, surface coating modification has emerged as an effective strategy to enhance graphite anode performance. This review systematically summarizes recent progress in coating materials (including carbon materials, lithium-ion conductors, metal compounds, and polymers) fabricated through vapor-phase or liquid-phase deposition. Enormous research investigations demonstrate that rationally designed coating layers prevent direct electrolyte/graphite contact to inhibit solvent decomposition, regulate lithium-ion flux distribution to promote uniform deposition, and function as artificial SEI components to improve interphasial stability. This review provides both theoretical insights and practical considerations for future research and development of advanced graphite anode materials for lithium-ion batteries.
- Graphite anode,
- Carbon anode,
- Surface coating,
- Solid-electrolyte interphase,
- Lithium-ion battery
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