Citation: Lewang Yuan, Yaoyao Peng, Zong-Jie Guan, Yu Fang. 二维共价有机框架作为光催化剂在有机合成中的研究进展[J]. Acta Physico-Chimica Sinica, ;2025, 41(8): 100086. doi: 10.1016/j.actphy.2025.100086 shu

二维共价有机框架作为光催化剂在有机合成中的研究进展

1.
College of Chemistry and Chemical Engineering, Hunan University, Changsha 410082, Hunan Province, China;
2.
State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou 350002, Fujian Province, China

Received Date: 11 February 2025
Revised Date: 18 March 2025
Accepted Date: 28 March 2025

Fund Project: This research was supported by National Natural Science Foundation of China (22371067).

二维共价有机框架(2D COFs)具有拓扑可调性、大比表面积、易于功能化以及出色的稳定性等特性，这些特性使得它们在多相光催化领域中的应用日益广泛。本文首先概述了2D COFs的合成方法，包括溶剂热、离子热、机械化学、微波辅助、声化学和界面合成方法。它简要介绍了影响光催化性能的各种因素，包括结晶度和稳定性、能带结构、电荷转移能力、孔径和比表面积以及光源。随后，讨论转向总结和分析2D COFs作为光催化剂在有机小分子转化反应(如光催化氧化、还原和偶联反应)中的进展。最后，对2D COFs在光催化有机转化领域面临的机遇和挑战进行了总结和展望。
- Two-dimension,
- Covalent organic framework,
- Photocatalysis,
- Oxidation reaction,
- Reduction reaction,
- Cross-coupling reaction
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