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二维共价有机框架作为光催化剂在有机合成中的研究进展

袁乐汪 ,  彭垚垚 ,  管宗杰 ,  方煜

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引用本文: 袁乐汪, 彭垚垚, 管宗杰, 方煜. 二维共价有机框架作为光催化剂在有机合成中的研究进展[J]. 物理化学学报, 2025, 41(8): 100086. doi: 10.1016/j.actphy.2025.100086 shu
Citation:  Lewang Yuan, Yaoyao Peng, Zong-Jie Guan, Yu Fang. Insights into the development of 2D covalent organic frameworks as photocatalysts in organic synthesis[J]. Acta Physico-Chimica Sinica, 2025, 41(8): 100086. doi: 10.1016/j.actphy.2025.100086 shu

二维共价有机框架作为光催化剂在有机合成中的研究进展

  • 1.

    湖南大学化学化工学院, 湖南 长沙 410082

  • 2.

    中国科学院福建物质结构研究所, 结构化学国家重点实验室, 福建 福州 350002

    • 通讯作者: 方煜, yu.fang@hnu.edu.cn
  • 基金项目:

    国家自然科学基金 22371067

摘要: 二维共价有机框架(2D COFs)具有拓扑可调性、大比表面积、易于功能化以及出色的稳定性等特性，这些特性使得它们在多相光催化领域中的应用日益广泛。本文首先概述了2D COFs的合成方法，包括溶剂热、离子热、机械化学、微波辅助、声化学和界面合成方法。它简要介绍了影响光催化性能的各种因素，包括结晶度和稳定性、能带结构、电荷转移能力、孔径和比表面积以及光源。随后，讨论转向总结和分析2D COFs作为光催化剂在有机小分子转化反应(如光催化氧化、还原和偶联反应)中的进展。最后，对2D COFs在光催化有机转化领域面临的机遇和挑战进行了总结和展望。

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