Citation: Yingtong Shi, Guotong Xu, Guizeng Liang, Di Lan, Siyuan Zhang, Yanru Wang, Daohao Li, Guanglei Wu. PEG-VN改性PP隔膜用于高稳定性高效率锂硫电池[J]. Acta Physico-Chimica Sinica, ;2025, 41(7): 100082. doi: 10.1016/j.actphy.2025.100082 shu

PEG-VN改性PP隔膜用于高稳定性高效率锂硫电池

1.
State Key Laboratory of Bio-fibers and Eco-textiles, College of Materials Science and Engineering, Qingdao University, Qingdao 266071, Shandong Province, China;
2.
Qingdao Engineering Research Center for New Metallic Functional Materials, Characteristic Laboratory of Advanced Metal Functional Materials and Processing in Universities of Shandong, Qingdao Binhai University, Qingdao 266555, Shandong Province, China;
3.
School of Automotive Materials, Hubei University of Automotive Technology, Shiyan 442002, Hubei Province, China;
4.
School of Chemistry and Chemical Engineering, Northwestern Polytechnical University, Xi'an 710072, Shaanxi Province, China

Received Date: 17 January 2025
Revised Date: 14 March 2025
Accepted Date: 18 March 2025

Fund Project: The project was supported by the National Natural Science Foundation of China (52302272, 52377026), Taishan Scholars and Young Experts Program of Shandong Province (tsqn202211124, tsqn202103057), the Natural Science Foundation of Shandong Province (ZR2022QB023, ZR2024ME046), the Qingchuang Talents Induction Program of Shandong Higher Education Institution (Research and Innovation Team of Marine Polysaccharides Fibers-based Energy Materials), the State Key Laboratory of Bio-Fibers and Eco-Textiles, Qingdao University (ZKT10, GZRC202006).

锂硫(Li-S)电池因其高理论能量密度被视为下一代能源存储系统中最有前景的候选者之一。然而，Li-S电池的实际应用受到锂离子(Li⁺)传输效率低和由于穿梭效应引起的快速容量衰减的限制。在此，我们报道了一种复合材料，由聚乙二醇(PEG)和氮化钒(VN)纳米片涂覆在商业聚丙烯(PP)隔膜上，称为PEG-VN@PP隔膜。VN纳米片所表现出的超催化效应和吸附特性显著增强了多硫化物的转化，从而提高了Li-S电池的容量和稳定性。由于PEG的涂层，Li⁺被极性官能团吸引，实现了选择性传输，改善了Li⁺的传输效率和Li-S电池的倍率性能。使用硫质量负载为1.2 mg·cm^-2的碳纳米管/硫阴极组装的Li-S电池，展现出高达782.0 mAh·g^-1的比容量，并在1C (1675 mA·g^-1)条件下经过700个循环后平均容量衰减为0.048%。
- Vanadium nitride,
- Polyethylene glycol,
- Separator modification,
- Shuttle effect,
- Lithium-sulfur batteries
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  南开大学师唯/华北电力大学（保定）刘景维：二维配位聚合物中有序的亲锂冠醚位点用于无枝晶锂沉积
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南开大学师唯/华北电力大学（保定）刘景维：二维配位聚合物中有序的亲锂冠醚位点用于无枝晶锂沉积

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