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Citation: Chao Liu, Huan Yu, Jiaming Li, Xi Yu, Zhuangzhi Yu, Yuxi Song, Feng Zhang, Qinfang Zhang, Zhigang Zou. 具有光热效应的多级Ti3C2/Bi12O17Br2肖特基异质结简单合成及其太阳能驱动抗生素光降解的研究[J]. Acta Physico-Chimica Sinica, ;2025, 41(7): 100075. doi: 10.1016/j.actphy.2025.100075 shu

具有光热效应的多级Ti3C2/Bi12O17Br2肖特基异质结简单合成及其太阳能驱动抗生素光降解的研究

  • 1.

    School of Materials Science and Engineering, Yancheng Institute of Technology, Yancheng 224051, Jiangsu Province, China

  • 2.

    Eco-Materials and Renewable Energy Research Centre (ERERC), Nanjing University, Nanjing 210093, Jiangsu Province, China

  • Corresponding author: Chao Liu, cliu@ycit.edu.cn Qinfang Zhang, qfangzhang@ycit.edu.cn
  • Received Date: 17 January 2025
    Revised Date: 24 February 2025
    Accepted Date: 3 March 2025

    Fund Project: the National Natural Science Foundation of Chin 12474276the National Natural Science Foundation of Chin 12274361

  • 在去除盐酸四环素(TC)方面，光催化技术被认为是一种高效和绿色的方法，可满足可持续发展的需求。本研究采用简单的搅拌过程来构建具有多级结构的Ti3C2/Bi12O17Br2 (命名为TBOB)肖特基异质结，其中Bi12O17Br2组分紧密地沉积在Ti3C2表面。通过模拟太阳光下降解TC来评价所有样品的光催化性能。与Bi12O17Br2相比，所制备的TBOB复合材料表现出更好的光降解活性，活性的增强归功于Ti3C2和Bi12O17Br2之间的协同效应，增加Ti3C2的负载量可提高光捕获能力，肖特基异质结的形成可促进有效的电荷载流子分离，以及光热效应可促进表面反应动力学。此外，对影响TBOB复合材料光催化性能的关键因素进行了详细的研究。自由基捕获实验和电子顺磁共振(EPR)技术证实了•O2−和e−是TC光催化降解的主要活性物种。结合实验分析和理论计算，提出并讨论了可能的电荷载流子转移途径和光催化降解机理。本研究为合理设计高效光热辅助Ti3C2基光催化剂提供了理论和实验依据。
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