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Citation: Fangxuan Liu, Ziyan Liu, Guowei Zhou, Tingting Gao, Wenyu Liu, Bin Sun. 中空结构光催化剂[J]. Acta Physico-Chimica Sinica, ;2025, 41(7): 100071. doi: 10.1016/j.actphy.2025.100071 shu

中空结构光催化剂

  • 1.

    Key Laboratory of Fine Chemicals in Universities of Shandong, Jinan Engineering Laboratory for Multi-Scale Functional Materials, School of Chemistry and Chemical Engineering, Qilu University of Technology (Shandong Academy of Sciences), Jinan 250353, Shandong Province, China

  • 2.

    Shandong Laboratory of Advanced Materials and Green Manufacturing at Yantai, Yantai 264006, Shandong Province, China

  • 3.

    Faculty of Mechanical Engineering, Qilu University of Technology (Shandong Academy of Sciences), Jinan 250353, Shandong Province, China

  • Corresponding author: Guowei Zhou, gwzhou@qlu.edu.cn Bin Sun, binsun@qlu.edu.cn
  • Received Date: 25 January 2025
    Revised Date: 19 February 2025
    Accepted Date: 24 February 2025

    Fund Project: the National Natural Science Foundation of China 52202102the National Natural Science Foundation of China 52472215the National Natural Science Foundation of China 52202007the National Natural Science Foundation of China 51972180Natural Science Foundation of Shandong Province ZR2019BB030Natural Science Foundation of Shandong Province ZR2021QE282Key Research & Development Project of Shandong Province 2024TSGC0222Science and Technology Support Plan for Youth Innovation of Colleges and Universities of Shandong Province 2021KJ056Science Fund of Shandong Laboratory of Advanced Materials and Green Manufacturing at Yantai AMGM2023F13Science Fund of Shandong Laboratory of Advanced Materials and Green Manufacturing at Yantai AMGM2021F05Science, Education and Industry Integration Innovation Pilot Project from Qilu University of Technology (Shandong Academy of Sciences) 2024ZDZX13

  • 利用太阳能驱动的光催化技术，有望成为缓解环境和能源压力的可行策略。因此，光催化性能的优异与否取决于光催化剂的合理设计。通过考虑形貌调控、带隙工程、助催化剂修饰以及异质结构建等因素，可以开发出性能优异的光催化剂。基于中空结构光催化剂独特特性的启发，具有中空结构的光催化剂在光催化剂设计中赋予了诸多优势，包括增强光的多重折射和反射、缩短光生载流子的传输距离以及提供丰富的表面反应位点。在此，我们系统地回顾了中空结构光催化剂的最新研究进展，并总结了其几何形貌、内部结构和化学成分的多样性。具体而言，我们重点介绍了中空结构光催化剂的合成策略，包括硬模板法、软模板法和无模板法。此外，还详细总结了一系列中空结构光催化剂，如金属氧化物、金属硫化物、金属有机框架和共价有机框架等。随后，我们概述了中空结构光催化剂在光催化污染物降解、H2生成、H2O2生成、CO2还原和N2固定等领域的潜在应用。同时，深入探讨了中空结构与光催化性能之间的内在关系。最后，我们分析了中空结构光催化剂未来发展方向中的挑战和前景。该综述为更好地设计中空结构光催化剂以满足环境修复和能源转换需求提供了启示。
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