Citation: Bing Han, Rui Lang, Botao Qiao, Aiqin Wang, Tao Zhang. Highlights of the major progress in single-atom catalysis in 2015 and 2016[J]. Chinese Journal of Catalysis, ;2017, 38(9): 1498-1507. doi: 10.1016/S1872-2067(17)62872-9 shu

Highlights of the major progress in single-atom catalysis in 2015 and 2016

Bing Han ^a,b, ,
Rui Lang ^a ,
Botao Qiao ^a ,
Aiqin Wang ^a ,
Tao Zhang ^a

a State Key Laboratory of Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, Liaoning, China;
b University of Chinese Academy of Sciences, Beijing 100049, China

Received Date: 24 April 2017
Revised Date: 7 June 2017

Fund Project: This work was supported by the National Natural Science Foundation of China (21606222, 21303184, 21573232), China Postdoctoral Science Foun-dation (2016M601350), Strategic Priority Research Program of the Chinese Academy of Sciences (XDB17020100), National Key Projects for Funda-mental Research and Development of China (2016YFA0202801), and Department of Science and Technology of Liaoning Province (2015020086-101).

The idea that single metal atoms dispersed on a solid support can act as an efficient heterogeneous catalyst was raised in 2011 when single Pt atoms on an FeO_x surface were reported to be active for CO oxidation and preferential oxidation of CO in H₂. The last six years have witnessed tremendous progress in the field of single-atom catalysis. Here we introduce the major achievements on this topic in 2015 and 2016. Some particular aspects of single-atom catalysis are discussed in depth, including new approaches in single-atom catalyst (SAC) synthesis, stable gold SACs for various reac-tions, the high selectivity of Pt and Pd SACs in hydrogenation, and the superior performance of non-noble metal SACs in electrochemistry. These accomplishments will encourage more efforts by researchers to achieve the controllable fabrication of SACs and explore their potential applications.
- Single-atom catalysis,
- Catalyst synthesis,
- CO oxidation,
- Hydrogenation,
- Electrocatalysis
1. [1]
2. [2]
3. [3]
4. [4]
5. [5]
6. [6]
7. [7]
8. [8]
9. [9]
10. [10]
11. [11]
12. [12]
13. [13]
14. [14]
15. [15]
16. [16]
17. [17]
18. [18]
19. [19]
20. [20]
21. [21]
22. [22]
23. [23]
24. [24]
25. [25]
26. [26]
27. [27]
28. [28]
29. [29]
30. [30]
31. [31]
32. [32]
33. [33]
34. [34]
35. [35]
36. [36]
37. [37]
38. [38]
39. [39]
40. [40]
41. [41]
42. [42]
43. [43]
44. [44]
45. [45]
46. [46]
47. [47]
48. [48]
49. [49]
50. [50]
51. [51]
52. [52]
53. [53]
54. [54]
55. [55]
56. [56]
57. [57]
58. [58]
59. [59]
60. [60]
61. [61]
62. [62]
63. [63]
64. [64]
65. [65]
66. [66]
67. [67]
68. [68]
69. [69]
70. [70]
71. [71]
72. [72]
73. [73]
74. [74]
75. [75]
76. [76]
77. [77]
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