Citation: Botao Qiao, Jin Xia Liang, Aiqin Wang, Jingyue Liu, Tao Zhang. Single atom gold catalysts for low-temperature CO oxidation[J]. Chinese Journal of Catalysis, ;2016, 37(10): 1580-1587. doi: 10.1016/S1872-2067(16)62529-9 shu

Single atom gold catalysts for low-temperature CO oxidation

a State Key Laboratory of Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, Liaoning, China;
b Guizhou Provincial Key Laboratory of Computational Nano-Material Science, Guizhou Education University, Guiyang 550018, Guizhou, China;
c Department of Physics, Arizona State University, Tempe, Arizona 85287, United States

Received Date: 1 June 2016
Revised Date: 23 August 2016

Fund Project: The authors acknowledge of the support by the National Natural Science Foundation of China (21303184, 21503046). J. Liang acknowledges the GZEU startup package. J. Liu acknowledges the support by the US National Science Foundation under CHE-1465057, Arizona State University, and the use of facilities in the John M. Cowley Center for High Resolution Electron Microscopy at Arizona State University. The authors also acknowledge the support by the Strategic Priority Research Program of the Chinese Academy of Sciences (XDB17020100) and the support by Department of Science and Technology of Liaoning Province (2015020086-101).

Low-temperature CO oxidation is important for both fundamental studies and practical applica-tions. Supported gold catalysts are generally regarded as the most active catalysts for low-temperature CO oxidation. The active sites are traditionally believed to be Au nanoclusters or nanoparticles in the size range of 0.5-5 nm. Only in the last few years have single-atom Au catalysts been proved to be active for CO oxidation. Recent advances in both experimental and theoretical studies on single-atom Au catalysts unambiguously demonstrated that when dispersed on suitable oxide supports the Au single atoms can be extremely active for CO oxidation. In this mini-review, recent advances in the development of Au single-atom catalysts are discussed, with the aim of illustrating their unique catalytic features during CO oxidation.
- Gold,
- Single atom catalyst,
- CO oxidation,
- Stability,
- Low temperature
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