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Citation: Siyu Lin, Linyan Yang, Xue Yang, Renxian Zhou. The effect of Pd precursor on Pd/Ce0.67Zr0.33O2 catalysts for automotive emission control[J]. Chinese Journal of Catalysis, ;2015, 36(4): 639-648. doi: 10.1016/S1872-2067(14)60264-3 shu

The effect of Pd precursor on Pd/Ce0.67Zr0.33O2 catalysts for automotive emission control

  • 1.

    Institute of Catalysis, Zhejiang University, Hangzhou 310028, Zhejiang, China

  • Corresponding author: Renxian Zhou, 
  • Received Date: 29 October 2014
    Available Online: 12 December 2014

    Fund Project: 国家高技术研究发展计划(863计划, 2011AA03A406) (863计划, 2011AA03A406) 浙江省重点科技创新团队计划(2009R50020). (2009R50020)

  • A Pd/CZ(NO) catalyst prepared with Pd(NO3)2 as the metal precursor exhibited the best catalytic performance for HC and CO elimination because of a higher oxygen storage capacity, abundant small Pdn clusters and a strong Pd-support interaction that facilitated electron transfer from PdOx particles to the CZ support. A Pd/CZ(NH) catalyst prepared with Pd(NH3)4(NO3)2 as the metal precursor exhibited good performance for NO and NO2 elimination due to a higher Pd dispersion, abundant bigger Pdn clusters and oxidized/metallic Pd coexistence. A Pd/CZ(Cl) catalyst prepared with H2PdCl4 as the metal precursor exhibited low catalytic activity due to a low Pd dispersion, weak Pd-support interaction, and the trace amount of CeOCl which inhibited oxygen vacancy creation. However, it showed good thermal stability, and benefited when an aging treatment removed the residual chlorine species and also promoted the interaction between PdOx and the support.
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